خيارات البحث
النتائج 1 - 10 من 352
Frequent algal blooms dramatically increase methane while decrease carbon dioxide in a shallow lake bay النص الكامل
2022
Zhang, Lei | He, Kai | Wang, Tong | Liu, Cheng | An, Yanfei | Zhong, Jicheng
Freshwater ecosystems play a key role in global greenhouse gas estimations and carbon budgets, and algal blooms are widespread owing to intensified anthropological activities. However, little is known about greenhouse gas dynamics in freshwater experiencing frequent algal blooms. Therefore, to explore the spatial and temporal variations in methane (CH₄) and carbon dioxide (CO₂), seasonal field investigations were performed in the Northwest Bay of Lake Chaohu (China), where there are frequent algal blooms. From the highest site in the nearshore to the pelagic zones, the CH₄ concentration in water decreased by at least 80%, and this dynamic was most obvious in warm seasons when algal blooms occurred. CH₄ was 2–3 orders of magnitude higher than the saturated concentration, with the highest in spring, which makes this bay a constant source of CH₄. However, unlike CH₄, CO₂ did not change substantially, and river mouths acted as hotspots for CO₂ in most situations. The highest CO₂ concentration appeared in winter and was saturated, whereas at other times, CO₂ was unsaturated and acted as a sink. The intensive photosynthesis of rich algae decreased the CO₂ in the water and increased dissolved oxygen and pH. The increase in CH₄ in the bay was attributed to the mineralization of autochthonous organic carbon. These findings suggest that frequent algal blooms will greatly absorb more CO₂ from atmosphere and increasingly release CH₄, therefore, the contribution of the bay to the lake's CH₄ emissions and carbon budget will be major even though it is small. The results of this study will be the same to other shallow lakes with frequent algal bloom, making lakes a more important part of the carbon budget and greenhouse gases emission.
اظهر المزيد [+] اقل [-]Attributed radiative forcing of air pollutants from biomass and fossil burning emissions النص الكامل
2022
Jiang, Ke | Fu, Bo | Luo, Zhihan | Xiong, Rui | Men, Yatai | Shen, Huizhong | Li, Bengang | Shen, Guofeng | Tao, Shu
Energy is vital to human society but significantly contributes to the deterioration of environmental quality and the global issue of climate change. Biomass and fossil fuels are important energy sources but have distinct pollutant emission characteristics during the burning process. This study aimed at attributing radiative forcing of climate forcers, including greenhouse gases but also short-lived climate pollutants, from the burning of fossil and biomass fuels, and the spatiotemporal characteristics. We found that air pollutant emissions from the burning process of biofuel and fossil fuels induced RFs of 68.2 ± 36.8 mW m⁻² and 840 ± 225 mW m⁻², respectively. The relatively contribution of biomass burning emissions was 7.6% of that from both fossil and biofuel combustion processes, while its contribution in energy supply was 11%. These relative contributions varied obviously across different regions. The per unit energy consumption of biomass fuel in the developed regions, such as North America (0.57 ± 0.33 mW m⁻²/10⁷TJ) and Western Europe (0.98 ± 0.79 mW m⁻²/10⁷TJ), had higher impacts of combustion emission related RFs compared to that of developing regions, like China (0.40 ± 0.26 mW m⁻²/10⁷TJ), and South and South-East Asia (0.31 ± 0.71 mW m⁻²/10⁷TJ) where low efficiency biomass burning in residential sector produced significant amounts of organic matter that had a cooling effect. Note that the study only evaluated fuel combustion emission related RFs, and those associated with the production of fuels and land use change should be studied later in promoting a comprehensive understanding on the climate impacts of biomass utilization.
اظهر المزيد [+] اقل [-]Comprehensive assessment of nitrous oxide emissions and mitigation potentials across European peatlands النص الكامل
2022
Lin, Fei | Zuo, Hongchao | Ma, Xiaohong | Ma, Lei
European natural peatlands have undergone long-term anthropogenic drainage activities that have severely decreased their functions, such as carbon sequestration. Recent rewetting has been conducted to restore the ecosystem services of peatlands and mitigate the emissions of potent greenhouse gases such as nitrous oxide (N₂O). However, the magnitudes and spatial patterns of annual N₂O fluxes and their mitigation potentials across European peatlands remain unknown. Here, we synthesized 492 annual N₂O flux data points from 77 in situ studies across European peatlands and found that the soil annual N₂O fluxes varied extensively from −1.08 to 33.40 kg N₂O–N ha⁻¹ yr⁻¹; these results were significantly and interactively (P < 0.05) affected by the peatland status, climatic regime and nutrient supply type. Drainage significantly (P < 0.05) stimulated soil N₂O emissions from natural minerotrophic rather than ombrotrophic peatlands, regardless of the climatic regime. Similarly, rewetting significantly (P < 0.05) reduced soil N₂O emissions from drained minerotrophic rather than ombrotrophic peatlands, demonstrating that the high N₂O emissions were driven by a simultaneous decline in the water table depth and increase in the soil nitrogen (N) availability. Magnitudes of the increases or decreases in N₂O emissions due to drainage or rewetting were also significantly influenced by the land-use and drainage history before rewetting and in the years following drainage/rewetting, respectively. The estimated annual mean N₂O emission total was found to be 90.42 (95% confidence interval: 64.49–122.57) Gg N₂O–N in 2020 from European peatlands. Scenario analysis showed that drained peatlands should be rewetted expeditiously; postponing rewetting would cause larger emissions from continued N₂O emissions from drained peatlands. Fully rewetting the drained peatlands used for forestry and peat extraction and partially rewetting those used for agriculture and grassland comprise a strategy for mitigating drained peatland N₂O emissions without compromising food security.
اظهر المزيد [+] اقل [-]Restored riverine wetlands in a headwater stream can simultaneously behave as sinks of N2O and hotspots of CH4 production النص الكامل
2021
Zhang, Wangshou | Li, Hengpeng | Pueppke, Steven G. | Pang, Jiaping
Wetlands can improve water quality, but they are also recognized as important sources of greenhouse gases (GHG) such as nitrous oxide (N₂O) and methane (CH₄). Emissions of these gases from wetland ecosystems, especially those in headwaters, are poorly understood. Here, we determined monthly concentrations of dissolved N₂O and CH₄ in a headwater stream of the Taihu Lake basin of China that contains both wetland and non-wetland reaches. Daily GHG dynamics in the wetland reach were also investigated. Riverine N₂O and CH₄ concentrations generally varied within 10–30 nmol L⁻¹ and 0.1–1.5 μmol L⁻¹, respectively. CH₄ saturation levels in the wetland reach were about seven times higher than those in the non-wetland reach, but there was no difference in N₂O saturation. In the wetland reach, saturation levels of CH₄ peaked in July, coincident with a dip in N₂O saturation to levels below its saturated solubility. This underscores that hotspots of CH₄ production and sinks for N₂O can occur occasionally in wetlands in mid-summer, when vegetative growth and microbial activities are high. Diurnal measurements indicated that CH₄ saturation in water flows passing through the wetlands from midnight through the early morning can surge to levels 10 times higher than those detected at other times of the day. Simultaneously, saturation levels of N₂O decreased by 75%, indicating a net consumption of N₂O. Changes in nutrient supply determined by upstream inflows, as well as dissolved oxygen, pH, and other environmental factors mediated by the wetlands, correlate with the differentiated behavior of N₂O and CH₄ production in wetlands. Additional work will be necessary to confirm the roles of these factors in regulating GHG emissions in riverine wetlands.
اظهر المزيد [+] اقل [-]Real-world particle and NOx emissions from hybrid electric vehicles under cold weather conditions النص الكامل
2021
Li, Chengguo | Swanson, Jacob | Pham, Liem | Hu, Shaohua | Hu, Shishan | Mikailian, Gary | Jung, Heejung S.
Hybrid electric vehicle (HEV) technology is critical to reduce the impact of the internal combustion engines on air pollution and greenhouse gases. HEVs have an advantage in market penetration due to their lower cost and higher driving range compared to battery electric vehicles (BEVs). On the other hand, HEVs use an internal combustion engine and still emit air pollutants. It is hypothesized that HEV performance is impacted by the weather conditions as a result of many factors. It was beyond the scope of this work to systematically evaluate all factors so instead we measured emissions from two vehicles driving city and highway routes in Minneapolis, Minnesota in the winter (−5 °C) and looked for major differences in emissions relative to each vehicle and relative to results that would be obtained from a chassis dynamometer in a controlled laboratory setting at a higher temperature approximately 20 °C). The study then looked to associate differences in emissions with the prevailing conditions to gain new insights. Emissions of interest included the total particle number (TPN), solid particle number (SPN), particulate matter mass (PM), and NOx. One key difference in vehicle engine technology was PFI (port fuel injection) versus GDI (gasoline direct injection). We found the frequency at which the Prius hybrid engine reignited was much higher than the Sonata for city and highway driving, although for both vehicles the catalyst temperature remained high and appeared to be unaffected by the reignitions, despite the cold weather. For most conditions, the Prius emitted more NOₓ but fewer particles than the Sonata. In some cases, NOₓ and particle emissions exceeded the most comparable laboratory-based emissions standards.
اظهر المزيد [+] اقل [-]Elucidating the impact of three metallic nanoagrichemicals and their bulk and ionic counterparts on the chemical properties of bulk and rhizosphere soils in rice paddies النص الكامل
2021
Growing applications of nanoagrichemicals have resulted in their increasing accumulation in agricultural soils, which could modify soil properties and affect soil health. A greenhouse pot trial was conducted to determine the effects of three metallic nanoagrichemicals on several fundamental chemical properties of a rice paddy soil, including zinc oxide nanoparticles (ZnO NPs) and copper oxide nanoparticles (CuO NPs) at 100 mg/kg, and silicon oxide nanoparticles (SiO₂ NPs) at 500 mg/kg, as well as their bulk and ionic counterparts. The investigated soil amendments displayed significant and distinctive impact on the examined soil chemical properties relevant to agricultural production, including soil pH, redox potential, soil organic carbon (SOC), cation exchange capacity (CEC), and plant available As. For example, all amendments increased the bulk soil pH at day 47 to some extent, but the increase was substantially higher for SiO₃²⁻ (37.7%) than other amendments (5.8%–13.7%). Soil Eh was elevated markedly at day 47 after the addition of soil amendments in both the bulk soil (45.9%–74.4%) and rice rhizosphere soil (20.3%–68.9%). CuO NPs and Cu²⁺ generally exhibited greater impact on soil chemical properties than other agrichemicals. Significantly different responses to soil amendments were observed between bulk and rhizosphere soils, suggesting the essential role of plants in affecting soil properties and their responses to environmental disturbance. Overall, our results confirmed that the tested amendments could have remarkable impacts on the fundamental chemical properties of rice paddy soils.
اظهر المزيد [+] اقل [-]Long-term trends in nitrogen oxides concentrations and on-road vehicle emission factors in Copenhagen, London and Stockholm النص الكامل
2021
Krecl, Patricia | Harrison, Roy M. | Johansson, Christer | Targino, Admir Créso | Beddows, David C. | Ellermann, Thomas | Lara, Camila | Ketzel, Matthias
Road transport is the main anthropogenic source of NOx in Europe, affecting human health and ecosystems. Thus, mitigation policies have been implemented to reduce on-road vehicle emissions, particularly through the Euro standard limits. To evaluate the effectiveness of these policies, we calculated NO₂ and NOx concentration trends using air quality and meteorological measurements conducted in three European cities over 26 years. These data were also employed to estimate the trends in NOx emission factors (EFNOₓ, based on inverse dispersion modeling) and NO₂:NOx emission ratios for the vehicle fleets under real-world driving conditions. In the period 1998–2017, Copenhagen and Stockholm showed large reductions in both the urban background NOx concentrations (−2.1 and −2.6% yr⁻¹, respectively) and EFNOₓ at curbside sites (68 and 43%, respectively), proving the success of the Euro standards in diminishing NOx emissions. London presented a modest decrease in urban background NOx concentrations (−1.3% yr⁻¹), while EFNOₓ remained rather constant at the curbside site (Marylebone Road) due to the increase in public bus traffic. NO₂ primary emissions —that are not regulated— increased until 2008–2010, which also reflected in the ambient concentrations. This increase was associated with a strong dieselization process and the introduction of new after-treatment technologies that targeted the emission reduction of other species (e.g., greenhouse gases or particulate matter). Thus, while regulations on ambient concentrations of specific species have positive effects on human health, the overall outcomes should be considered before widely adopting them. Emission inventories for the on-road transportation sector should include EFNOₓ derived from real-world measurements, particularly in urban settings.
اظهر المزيد [+] اقل [-]Paddy-upland rotation with Chinese milk vetch incorporation reduced the global warming potential and greenhouse gas emissions intensity of double rice cropping system النص الكامل
2021
Zhong, Chuan | Liu, Ying | Xu, Xintong | Yang, Binjuan | Aamer, Muhammad | Zhang, Peng | Huang, Guoqin
It is a common practice to maintain soil fertility based on the paddy-upland rotation with green manure in the subtropical region of China. However, rare studies are known about greenhouse gas (GHG) emissions from the paddy-upland rotation with green manure incorporation. Therefore, we conducted a field experiment of two years to compared with the effect of two kinds of green manure (CV: Chinese milk vetch and OR: Oilseed rape), and two kinds of cropping system (DR: double rice system and PR: paddy-upland rotation) on greenhouse gases emissions. We have found that the annual accumulation of CH₄ of Chinese milk vetch-rice-sweet potato || soybean was significantly reduced by 32.95%∼63.22% compared with other treatments, mainly because Chinese milk vetch reduced the abundance of methanogens by reducing soil C/N ratio. Meanwhile increasing soil permeability resulting from paddy-upland rotation also reduced soil CH₄ emission. However, The annual accumulation of N₂O of Chinese milk vetch-rice-sweet potato || soybean was increased by 17.39%∼870.11% compared with other treatments, mainly attributed to paddy-upland rotation decreased soil pH and nosZ abundance and increased nirK and nirS, thus enhancing N₂O emission, meanwhile the Chinese milk vetch incorporation and its interaction with the paddy-upland rotation has greatly enhanced the contents of NO₃⁻-N and abundance of ammonia-oxidizing archaea (AOA). The area-scaled global warming potential (GWP) and the biomass-scaled greenhouse gas emissions intensity (GHGI) of Chinese milk vetch-rice-sweet potato || soybean was reduced by 19.01%∼50.69% and 5.38%∼35.77% respectively. Thereby, the Chinese milk vetch-rice-sweet potato || soybean cropping system was suitable for agricultural sustainable development.
اظهر المزيد [+] اقل [-]Eco-friendly yield-scaled global warming potential assists to determine the right rate of nitrogen in rice system: A systematic literature review النص الكامل
2021
Islam Bhuiyan, Mohammad Saiful | Rahamāna, Ājijura | Kim, Gil Won | Das, Suvendu | Kim, Pil Joo
Rice paddies are one of the largest greenhouse gases (GHGs) facilitators that are predominantly regulated by nitrogen (N) fertilization. Optimization of N uses based on the yield has been tried a long since, however, the improvement of the state-of-the-art technologies and the stiffness of global warming need to readjust N rate. Albeit, few individual studies started to, herein attempted as a systematic review to generalize the optimal N rate that minimizes global warming potential (GWP) concurrently provides sufficient yield in the rice system. To satisfy mounted food demand with inadequate land & less environmental impact, GHGs emissions are increasingly evaluated as yield-scaled basis. This systematic review (20 published studies consisting of 21 study sites and 190 observations) aimed to test the hypothesis that the lowest yield-scaled GWP would provide the minimum GWP of CH₄ and N₂O emissions from rice system at near optimal yields. Results revealed that there was a strong polynomial quadratic relationship between CH₄ emissions and N rate and strong positive correlation between N₂O emissions and N rate. Compared to control the low N dose emitted less (23%) CH₄ whereas high N dose emitted higher (63%) CH₄ emission. The highest N₂O emission observed at moderated N level. In total GWP, about 96% and 4%, GHG was emitted as CH₄ and N₂O, respectively. The mean GWP of CH₄ and N₂O emissions from rice was 5758 kg CO₂ eq ha⁻¹. The least yield-scaled GWP (0.7565 (kg CO₂ eq. ha⁻¹)) was recorded at 190 kg N ha⁻¹ that provided the near utmost yield. This dose could be a suitable dose in midseason drainage managed rice systems especially in tropical and subtropical climatic conditions. This yield-scaled GWP supports the concept of win–win for food security and environmental aspects through balancing between viable rice productivity and maintaining convincing greenhouse gases.
اظهر المزيد [+] اقل [-]Fuel consumption and air emissions in one of the world’s largest commercial fisheries النص الكامل
2021
Chassot, Emmanuel | Antoine, Sharif | Guillotreau, Patrice | Lucas, Juliette | Assan, Cindy | Marguerite, Michel | Lamboy, Nathalie Bodin
Fuel consumption and air emissions in one of the world’s largest commercial fisheries النص الكامل
2021
Chassot, Emmanuel | Antoine, Sharif | Guillotreau, Patrice | Lucas, Juliette | Assan, Cindy | Marguerite, Michel | Lamboy, Nathalie Bodin
The little information available on fuel consumption and emissions by high seas tuna fisheries indicates that the global tuna fleet may have consumed about 2.5 Mt of fuel in 2009, resulting in the production of about 9 Mt of CO₂-equivalent greenhouse gases (GHGs), i.e., about 4.5–5% of the global fishing fleet emissions. We developed a model of annual fuel consumption for the large-scale purse seiners operating in the western Indian Ocean as a function of fishing effort, strategy, and vessel characteristics based on an original and unique data set of more than 4300 bunkering operations that spanned the period 2013–2019. We used the model to estimate the total fuel consumption and associated GHG and SO₂ emissions of the Indian Ocean purse seine fishery between 1981 and 2019. Our results showed that the energetic performance of this fishery was characterized by strong interannual variability over the last four decades. This resulted from a combination of variations in tuna abundance but also changes in catchability and fishing strategy. In recent years, the increased targeting of schools associated with fish aggregating devices in response to market incentives combined with the IOTC management measure implemented to rebuild the stock of yellowfin tuna has strongly modified the productivity and spatio-temporal patterns of purse seine fishing. This had effects on fuel consumption and air pollutant emissions. Over the period 2015 to 2019, the purse seine fishery, including its support vessel component, annually consumed about 160,000 t of fuel and emitted 590,000 t of CO2-eq GHG. Furthermore, our results showed that air pollutant emissions can be significantly reduced when limits in fuel composition are imposed. In 2015, SO₂ air pollution exceeded 1500 t, but successive implementation of sulphur limits in the Indian Ocean purse seine fishery in 2016 and 2018 have almost eliminated this pollution. Our findings highlight the need for a routine monitoring of fuel consumption with standardized methods to better assess the determinants of fuel consumption in fisheries and the air pollutants they emit in the atmosphere.
اظهر المزيد [+] اقل [-]Fuel consumption and air emissions in one of the world’s largest commercial fisheries النص الكامل
2021
Chassot, Emmanuel | Antoine, Sharif | Guillotreau, Patrice | Lucas, Juliette | Assan, Cindy | Marguerite, Michel | Bodin, Nathalie
The little information available on fuel consumption and emissions by high seas tuna fisheries indicates that the global tuna fleet may have consumed about 2.5 Mt of fuel in 2009, resulting in the production of about 9 Mt of CO2-equivalent greenhouse gases (GHGs), i.e., about 4.5–5% of the global fishing fleet emissions. We developed a model of annual fuel consumption for the large-scale purse seiners operating in the western Indian Ocean as a function of fishing effort, strategy, and vessel characteristics based on an original and unique data set of more than 4300 bunkering operations that spanned the period 2013–2019. We used the model to estimate the total fuel consumption and associated GHG and SO2 emissions of the Indian Ocean purse seine fishery between 1981 and 2019. Our results showed that the energetic performance of this fishery was characterized by strong interannual variability over the last four decades. This resulted from a combination of variations in tuna abundance but also changes in catchability and fishing strategy. In recent years, the increased targeting of schools associated with fish aggregating devices in response to market incentives combined with the IOTC management measure implemented to rebuild the stock of yellowfin tuna has strongly modified the productivity and spatio-temporal patterns of purse seine fishing. This had effects on fuel consumption and air pollutant emissions. Over the period 2015 to 2019, the purse seine fishery, including its support vessel component, annually consumed about 160,000 t of fuel and emitted 590,000 t of CO2-eq GHG. Furthermore, our results showed that air pollutant emissions can be significantly reduced when limits in fuel composition are imposed. In 2015, SO2 air pollution exceeded 1500 t, but successive implementation of sulphur limits in the Indian Ocean purse seine fishery in 2016 and 2018 have almost eliminated this pollution. Our findings highlight the need for a routine monitoring of fuel consumption with standardized methods to better assess the determinants of fuel consumption in fisheries and the air pollutants they emit in the atmosphere.
اظهر المزيد [+] اقل [-]