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Cadmium and associated metals in soils and sediments of wetlands across the Northern Plains, USA
2013
Jacob, Donna L. | Yellick, Alex H. | Kissoon, La Toya T. | Asgary, Aida | Wijeyaratne, Dimuthu N. | Saini-Eidukat, Bernhardt | Otte, Marinus L.
Cadmium, present locally in naturally high concentrations in the Northern Plains of the United States, is of concern because of its toxicity, carcinogenic properties, and potential for trophic transfer. Reports of natural concentrations in soils are dominated by dryland soils with agricultural land uses, but much less is known about cadmium in wetlands. Four wetland categories – prairie potholes, shallow lakes, riparian wetlands, and river sediments – were sampled comprising more than 300 wetlands across four states, the majority in North Dakota. Cd, Zn, P, and other elements were analyzed by ICP-MS, in addition to pH and organic matter (as loss-on-ignition). The overall cadmium content was similar to the general concentrations in the area's soils, but distinct patterns occurred within categories. Cd in wetland soils is associated with underlying geology and hydrology, but also strongly with concentrations of P and Zn, suggesting a link with agricultural land use surrounding the wetlands.
اظهر المزيد [+] اقل [-]Associations between environmental pollutants and larval amphibians in wetlands contaminated by energy-related brines are potentially mediated by feeding traits
2019
Smalling, Kelly L. | Anderson, Chauncey W. | Honeycutt, R Ken | Cozzarelli, Isabelle M. | Preston, Todd | Hossack, Blake R.
Energy production in the Williston Basin, located in the Prairie Pothole Region of central North America, has increased rapidly over the last several decades. Advances in recycling and disposal practices of saline wastewaters (brines) co-produced during energy production have reduced ecological risks, but spills still occur often and legacy practices of releasing brines into the environment caused persistent salinization in many areas. Aside from sodium and chloride, these brines contain elevated concentrations of metals and metalloids (lead, selenium, strontium, antimony and vanadium), ammonium, volatile organic compounds, hydrocarbons, and radionuclides. Amphibians are especially sensitive to chloride and some metals, increasing potential effects in wetlands contaminated by brines. We collected bed sediment and larval amphibians (Ambystoma mavortium, Lithobates pipiens and Pseudacris maculata) from wetlands in Montana and North Dakota representing a range of brine contamination history and severity to determine if contamination was associated with metal concentrations in sediments and if metal accumulation in tissues varied by species. In wetland sediments, brine contamination was positively associated with the concentrations of sodium and strontium, both known to occur in oil and gas wastewater, but negatively correlated with mercury. In amphibian tissues, selenium and vanadium were associated with brine contamination. Metal tissue concentrations were higher in tadpoles that graze compared to predatory salamanders; this suggests frequent contact with the sediments could lead to greater ingestion of metal-laden materials. Although many of these metals may not be directly linked with energy development, the potential additive or synergistic effects of exposure along with elevated chloride from brines could have important consequences for aquatic organisms. To effectively manage amphibian populations in wetlands contaminated by saline wastewaters we need a better understanding of how life history traits, species-specific susceptibilities and the physical-chemical properties of metals co-occurring in wetland sediments interact with other stressors like chloride and wetland drying.
اظهر المزيد [+] اقل [-]Does Increased Road Dust Due to Energy Development Impact Wetlands in the Bakken Region?
2016
Creuzer, Jessica | Hargiss, Christina L. M. | Norland, Jack E. | DeSutter, Thomas | Casey, Francis X. | DeKeyser, Edward S. | Ell, Mike
The Bakken region of western North Dakota and Montana from January 2012 to December 2013 saw an increase of 3368 oil wells, causing a major increase in road dust emissions. A portion of the energy extraction in the Bakken occurs in the wetland rich Prairie Pothole Region, and there is little information on gravel road dust emissions or the ecological impacts. The objectives of this study were to (1) estimate surface loading of gravel road dust during different times of year and at different distances from the road, (2) evaluate dust loading effects on surface water quality, and (3) evaluate the impact of dust deposition on wetland soils. Ten wetlands were tested in the energy impacted area and ten in an adjacent area without energy development. There was a 355 % increase in dust loading 10 m from the road in the energy impacted area compared to an area without energy development; meanwhile, there was only a 46 % increase in dust loading 40 m from the road. This loading resulted in an annual deposition of 647 g/m² of gravel road dust close to the road. However, the effect of dust loading on the water quality and soils of wetlands was minimal when compared to wetlands not impacted by increased gravel road dust. The finding of minimal effect on wetland resources from increased road dust fills a knowledge gap in the Bakken on how energy development alters the environment.
اظهر المزيد [+] اقل [-]Sediment-bound Arsenic and Uranium Within the Bowman–Haley Reservoir, North Dakota
2011
Larson, Lance N. | Stone, James J.
The purpose of this study was to determine the impacts of regional historical uranium mining activities within sediments of the Bowman–Haley reservoir of southwestern North Dakota. The extent of anthropogenic-influenced watershed impacts were quantified through the determination of sediment metals concentrations and metal enrichment factors to evaluate the potential of geochemically influenced As and U remobilization within the reservoir sediments. Sediment cores were collected and analyzed for total metal concentrations at five locations within the reservoir: Spring Creek delta, Alkali Creek delta, two locations within the North Fork of the Grand River confluence, and adjacent to the reservoir outfall. Pearson-moment correlations were used to establish inter-core metal correlations, while sediment enrichment factors were determined relative to background concentrations. Enrichment factor results suggest all sampling sites are classified as minor to moderately enriched for As and U. Metal behavior for the three reservoir inlets indicated similar metal loading sources and post-depositional behavior, while metals migration within the vicinity of the reservoir outlet appear to be controlled by geochemical and/or physical processes. For the reservoir outlet, As and U normalized to Al suggest the occurrence of vertical migration of As, while surface-bound U remobilization was apparent within the water column immediately above the sediments. Elevated U was found within the Spring Creek inlet, and appear attributed to historical uranium processing operations located in Griffin, North Dakota. While the reservoir As and U sediment concentrations may be considered low, their presence appears directly attributed to historical uranium mining activities within the Bowman–Haley reservoir watershed.
اظهر المزيد [+] اقل [-]The shale gas production and economic growth in local economies across the US
2020
Bilgili, Faik | Koçak, Emrah | Bulut, Ümit
Recently, several seminal works have been drawing attention to the revolution of shale gas production technology of the USA, the impact of shale gas on energy sectors, as well as the influences of shale gas on macroeconomic variables of employment, economic growth, etc. Nevertheless, one may claim that two gaps appear in literature. The first gap is the absence of an econometric study estimating the effect of shale oil/gas on national economies. The more considerable second gap is the absence of econometric analyses revealing the impulses of shale gas on local economies. Therefore, this paper observes the possible causalities between the shale gas and local gross domestic product (GDP) employing quarterly data covering the period 2007–2016 for 12 states in the US. After performing the tests of cross-sectional dependence, heterogeneity, stationarity, and cointegration, the paper conducts the panel Granger causality analyses. The empirical findings depict that (i) there is available unidirectional relationship from local shale gas production to local GDP in Colorado, Ohio, and West Virginia; (ii) there occurs an impulse from GDP to local shale gas production for Louisiana, North Dakota, and Oklahoma; (iii) a bidirectional causality coexists between local shale gas production and GDP in Arkansas, California, and Texas; and (iv) there exists no association between local GDP and local shale gas extraction in Montana, New Mexico, and Wyoming.
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