Total Synthesis of (−)-Lepenine
2014
Nishiyama, Yoshitake | Han-ya, Yuki | Yokoshima, Satoshi | Fukuyama, Tohru
The first asymmetric total synthesis of lepenine has been accomplished. The synthesis features a tethered intramolecular Diels–Alder reaction, an intramolecular Mannich reaction, and a Diels–Alder reaction between an ortho-quinone monoketal and ethylene, resulting in stereoselective construction of the unique hexacyclic system.
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