Selective adsorption and separation of C₂ hydrocarbons in a “flexible-robust” metal–organic framework based on a guest-dependent gate-opening effect
2020
Zhang, Peng-Dan | Wu, Xue-Qian | He, Tao | Xie, Lin-Hua | Chen, Qiang | Li, Jian Rong
The selective adsorption/separation of C₂ hydrocarbons has been realized in a “flexible-robust” MOF, Zn₂(Atz)₂Ox. Owing to the distinctive guest-dependent multistep adsorption behaviors and suitable guest–framework interactions, this MOF shows outstanding separation performance for C₂H₂/C₂H₄ mixtures in a wide range of temperature confirmed by a column breakthrough experiment.
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