Thermodynamics and kinetics of CO₂, CO, and H⁺ binding to the metal centre of CO₂ reduction catalysts
2012
Schneider, Jacob | Jia, Hongfei | Muckerman, James T. | Fujita, Etsuko
In our developing world, carbon dioxide has become one of the most abundant greenhouse gases in the atmosphere. It is a stable, inert, small molecule that continues to present significant challenges toward its chemical activation as a useful carbon end product. This tutorial review describes one approach to the reduction of carbon dioxide to carbon fuels, using cobalt and nickel molecular catalysts, with particular focus on studying the thermodynamics and kinetics of CO₂ binding to metal catalytic sites.
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