Surface confined self-assembly of polyampholytes generated from charge-shifting polymers
2015
Garnier, T. | Dochter, A. | Chau, N. T. T. | Schaaf, P. | Jierry, L. | Boulmedais, F.
Polyampholyte-based films can be efficiently self-assembled onto a surface in a one-pot manner. By using a gradient of protons, morphogens, generated at an electrode surface, a charge-shifting polyelectrolyte present in solution can be transformed into a polyampholyte, leading to the continuous buildup of a film based on polyelectrolyte complexation.
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