Recovery of Clean Water and Ammonia from Domestic Wastewater: Impacts on Embodied Energy and Greenhouse Gas Emissions
2022
Shin, Chungheon | Szczuka, Aleksandra | Liu, Matthew J. | Mendoza, Lorelay | Jiang, Renjing | Tilmans, Sebastien H. | Tarpeh, William A. | Mitch, William A. | Criddle, Craig S.
Treatment of domestic wastewater can recover valuable resources, including clean water, energy, and ammonia. Important metrics for these systems are greenhouse gas (GHG) emissions and embodied energy, both of which are location- and technology-dependent. Here, we determine the embodied energy and GHG emissions resulting from a conventional process train, and we compare them to a nonconventional process train. The conventional train assumes freshwater conveyance from a pristine source that requires energy for pumping (US average of 0.29 kWh/m³), aerobic secondary treatment with N removal as N₂, and Haber-Bosch synthesis of ammonia. Overall, we find that this process train has an embodied energy of 1.02 kWh/m³ and a GHG emission of 0.77 kg-CO₂eq/m³. We compare these metrics to those of a nonconventional process train that features anaerobic secondary treatment technology followed by further purification of the effluent by reverse osmosis and air stripping for ammonia recovery. This “short-cut” process train reduces embodied energy to 0.88 kWh/m³ and GHG emissions to 0.42 kg-CO₂eq/m³, while offsetting demand for ammonia from the Haber-Bosch process and decreasing reliance upon water transported over long distances. Finally, to assess the potential impacts of nonconventional nitrogen removal technology, we compared the embodied energy and GHG emissions resulting from partial nitritation/anammox coupled to anaerobic secondary treatment. The resulting process train enabled a lower embodied energy but increased GHG emissions, largely due to emissions of N₂O, a potent greenhouse gas.
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