Distribution and Sources of Heavy Metals in Stormwater: Influence of Land Use in Camden, New Jersey

Heavy metals are widespread environmental contaminants from natural and anthropogenic sources, posing risks to human health and ecosystems. In urban areas, levels are elevated due to industrial activity, traffic emissions, and building materials. Camden, New Jersey, a city with a history of industry and illegal dumping, faces increased risk due to aging sewer and stormwater systems. These systems frequently flood neighborhoods and parks, heightening residents&rsquo: exposure to heavy metals. Despite this, few studies have examined metal distribution in Camden, particularly during storm events. This study analyzes stormwater metal concentrations across residential and commercial areas to assess contamination levels, potential sources, and land use associations. Stormwater samples were collected from 33 flooded street locations after four storm events in summer 2023, along with samples from a flooded residential basement during three storms. All were analyzed for total lead, cadmium, and arsenic using inductively coupled plasma&ndash:mass spectrometry (ICP-MS, (Department of Chemistry and Biochemistry, Rowan University, Glassboro, NJ, USA)). Concentration data were visualized using geographic information system (GIS)-based mapping in relation to land use, socioeconomic, and public health factors. In Camden&rsquo:s stormwater, lead levels (1&ndash:1164 &micro:g L&minus:1) were notably higher than those of cadmium (0.1&ndash:3.3 &micro:g L&minus:1) and arsenic (0.2&ndash:8.6 &micro:g L&minus:1), which were relatively low. Concentrations varied citywide, with localized hot spots shaped by environmental and socio-economic factors. Principal component analysis indicates lead and cadmium likely originate from shared sources, mainly industries and illegal dumping. Notably, indoor stormwater samples showed higher heavy metal concentrations than outdoor street samples, indicating greater exposure risks in flooded homes. These findings highlight the spatial variability and complex sources of heavy metal contamination in stormwater, underscoring the need for targeted interventions in vulnerable communities.