In 1985-99 studies were carried out in the area of the Kunda cement plant on North Estonian coastal plain on sample plots stretching 1.5 and 2.5 km east and 2 km and 3 km west, where changes in crown damages and radial increment of pine and spruce were estimated. The selected stands were with 0.7-0.8 density and II quality class, with moderately dense or sprase understorey, 75-85-year-old Myrtillus site type pine or spruce stands. Practically every tree in the area of intensive dust pollution had signs of damage. The relations between the defoliation and radial increment in the region were not linear. Weak defoliation (up to 25 per cent) influences slightly the radial growth. The correlations were more evident on Pinus sylvestris with more than half of the trees in the area having moderate or strong defoliation (at least 30-35 per cent). We suppose that defoliation, which leads to a decrease in the assimilating area of trees, causes essential changes in physiological processes. In the region of intensive pollution stress the radial increment decreased along with the defoliation level on both Pinus sylvestris and Picea abies

The influence of air pollution from a cement plant on chlorophylls and carotenoids of the needles of Scots pine and Norway spruce was studied on the sample plots established at different distances from the emission centre in 1992, 1994 and 1999. No essential difference was observed in pigment concentrations in needles between 1992, when the emission of cement dust from the plant was very high, and 1999, when dust pollution had practically stopped. The negative influence on the synthesis of pigments in needles occurred through the alkalisation of soil and disbalances of mineral nutrients accumulation into the organism

The present paper is based on experiments carried out with black spruce in the industrial area North-East Estonia. Two-year-old seedlings of black spruce were planted in a sample plot affected by a cement plant and by oil-shale processing enterprises and in an unpolluted control sample plot in 1990. At the end of the experiment in 1997 it was ascertained that the impact of industrial alkaline air pollution complexes resulting in the alkalisation and chemical deviations of growth conditions retards the height growth of trees and brings about a decrease in their biomass. The sturdiness quotient was higher and the Dickson quality index was lower than the control, indicating serious damages of trees under air pollution. Increasing share of needles in the total biomass in polluted areas in comparison with control trees suggest that compensation mechanism were started in trees to increase the assimilating mass in order to survive under stress. The state of young black spruces in alkalised industrial areas shows unsuitability of using this species in industrial areas

Element concentrations in the xylem wood of Scots pines (Pinus sylvestris L.) growing in different soil and pollution load conditions at Narva-Joesuu and Haeaedemeeste, Estonia, were studied for temporal trends with respect to soil properties. The upper horizons of the Haeaedemeeste stand soil profile were strongly acidic compared with those of Narva-Joesuu, which were weakly acidic. Element concentrations for K, Ca, Mg, Mn and Zn in upper soil horizons were higher at the Narva-Joesuu stand and for Pb at Haeaedemeeste. Concentrations of xylem elements Mg, K, P, Pb and Cu were higher in the Narva-Joesuu sample and of Ca, Mn and Zn in the Haeaedemeeste sample. The concentrations of xylem elements except for K, Mg and Cu were poorly associated with those in soil. The increasing concentrations of Ca, K, P and in the Narva-Joesuu sample during the last decades can be explained by the larger amounts of emissions of the oil-shale fly ash by the neighbouring thermal electric power stations. Thus, the alteration of the concentrations of these elements in the xylem offer a promise for determining deposition-mediated changes in the environment

To study the impact of air pollution on the growth of conifers sample plots were established at different distances and directions from the Kunda cement plant. The plots included stands of 70-80-year-old Scots pine and Norway spruce. Although emission of alkaline cement dust had decreased in the second half of the 1990s analyses of soil samples collected to characterise the growth substrate of trees showed that the pH value of the humus horizon of weakly podzolised temporarily overmoist sandy soils was within the radius of 3 km from the cement plant 2.0-2.9 times as high as that of the control plots in Lahemaa National Park. To ascertain the effect of alkaline environment on the growth of conifers the length (cm) of the needles and shoots formed in 1996-99, dry and wet mass (g) of 100 needles, dry matter content of needles(per cent) and density of needles on shoots were measured. The results obtained were compared with data from 1992 if possible. Both pine and spruce were found to be sensitive towards cement dust pollution and alkalised environment; however, the impact on different morphological parameters was different. As compared to the control, the strongest inhibition of growth was revealed in the sample plot situated 2.5 km east from the cement plant. Conifers on sample plots 2 km west from the emission source showed more vigorous growth than the control. As compared with data from 1992, some improvement in the growth of pine and spruce was observed

The greatest sources of atmospheric emissions of alkaline dust and SO2 in Estonia are the soil shale based power plants and the cement production. In the vicinity of oil sale processing and chemical plants the organic pollutants, as well asammonia, H2S etc. are also found in the ambient air. Temporal changes in emission amounts and in atmospheric air pollution levels in North-East Estonia since 1960 until today (1997-98) are discussed. During the period of 1989-98 the emissions from power plants decreased about 2.5 times and those from cement production up to 40 times. In 1960-89 oil shale fly ash was the prevalent factor of air pollution, most notably in north-eastern and northern parts of the region. Since 1990-91 the proportion of SO2 has increased in the balance of alkaline and acidic components in some industrial areas. Zonation of landscapes on the basis of air pollution and the critical loads of pollutants for forest trees and Sphagnum are discussed

Forty-five macrolichen species were registered on 29 forested sample plots in Laeaene- and Ida-Viru counties in North-East Estonia. Analysis of the macrolichen species distribution indicated and impact of air pollution on the epiphytic lichen cover. The presented distribution maps demonstrate that lichen species belonging to different ecological groups by substrate requirements respond differently to air pollution. Lichen species diversity was analysed by means of species richness, diferent diversity measures including the Shannon-Weaver Diversity Index, and characterised by the sum of species abundances. Alpha diversity of epiphytic macrolichens for the study area is 8.3 (s.d. 5.5), beta diversity 5.4, and the Shannon-Weaver Diversity Index varied from 0 to 1.189. Variations in the lichen community demonstrated the existence of a steep local air pollution gradient oriented from north-east to south-west

It was ascertained that the content of soluble sugars, starch and ratios between different forms of carbohydrates varied in the trees growing in areas affected by industrial production in Kohtla-Jaerve and Kunda. The ratio of soluble sugars to starch is a good indicator of the state of trees in industrial areas. This ratio depends on the level of air pollution. In the studied areas a strong relationship between the content of soluble sugars and N, Mg and K was observed in the needles of Norway spruce

The research was conducted in 1990-99 in forest observation sites in the neighbourhoods of industrial enterprises of Kohtla-Jaerve-Johvi and the cement plant of Kunda and in the control area in Lahemaa National Park. Differences between the radial increments of conifers growing under pollution and in a relatively unpolluted area were estimated. The stands selected for investigation were similar as to their edaphic conditions and forest survey indicators. The high sensitivity of conifers to long term emissions of pollutants into the atmosphere from oil shale based power engineering and chemical industry, production of building materials and fertilisers and other industrial enterprises in the investigation area is expressed as changes in the radial increment of trees with the changes depending on the pollution load and alterations in precipitation and soil

Prolonged effects of the multicomponent air pollution complexes emitted from the cement production in Kunda and oil shale processing in Kohtla-Jaerve, North-East estonia, on the forest ecosystems are discussed. It was found that atmospheric input substantially affects biogeochemical cycling in forest. The comparatively high concentrations of alkaline dusts and ash and various gaseous pollutants in the atmosphere of the investigated areas over 40 years have caused qualitative and quantitative changes in the forest soil, soil water and precipitation and in the state of forest and trees. Although the levels of air pollutants emitted by the industry have seriously decreased in recent years, alkalisation of the growth environment of trees is still essential in some regions. Alkalisation of soil and soil water in the vicinity of Kunda and Kohtla-Jaerve complicated mineral nutrition processes and disbalanced mineral elements composition in tissues, which resulted in a decrease in the increment and quality of trees