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Sources, distribution and export coefficient of phosphorus in lowland polders of Lake Taihu Basin, China
2017
Huang, Jiacong | Gao, Junfeng | Jiang, Yong | Yin, Hongbin | Amiri, Bahman Jabbarian
Identifying phosphorus (P) sources, distribution and export from lowland polders is important for P pollution management, however, is challenging due to the high complexity of hydrological and P transport processes in lowland areas. In this study, the spatial pattern and temporal dynamics of P export coefficient (PEC) from all the 2539 polders in Lake Taihu Basin, China were estimated using a coupled P model for describing P dynamics in a polder system. The estimated amount of P export from polders in Lake Taihu Basin during 2013 was 1916.2 t/yr, with a spatially-averaged PEC of 1.8 kg/ha/yr. PEC had peak values (more than 4.0 kg/ha/yr) in the polders near/within the large cities, and was high during the rice-cropping season. Sensitivity analysis based on the coupled P model revealed that the sensitive factors controlling the PEC varied spatially and changed through time. Precipitation and air temperature were the most sensitive factors controlling PEC. Culvert controlling and fertilization were sensitive factors controlling PEC during some periods. This study demonstrated an estimation of PEC from 2539 polders in Lake Taihu Basin, and an identification of sensitive environmental factors affecting PEC. The investigation of polder P export in a watershed scale is helpful for water managers to learn the distribution of P sources, to identify key P sources, and thus to achieve best management practice in controlling P export from lowland areas.
Show more [+] Less [-]Three-dimensional investigation of ozone pollution in the lower troposphere using an unmanned aerial vehicle platform
2017
Li, Xiao-Bing | Wang, Dong-Sheng | Lu, Qing-Chang | Peng, Zhong-Ren | Lu, Si-Jia | Li, Bai | Li, Chao
Potential utilities of instrumented lightweight unmanned aerial vehicles (UAVs) to quickly characterize tropospheric ozone pollution and meteorological factors including air temperature and relative humidity at three-dimensional scales are highlighted in this study. Both vertical and horizontal variations of ozone within the 1000 m lower troposphere at a local area of 4 × 4 km² are investigated during summer and autumn times. Results from field measurements show that the UAV platform has a sufficient reliability and precision in capturing spatiotemporal variations of ozone and meteorological factors. The results also reveal that ozone vertical variation is mainly linked to the vertical distribution patterns of air temperature and the horizontal transport of air masses from other regions. In addition, significant horizontal variations of ozone are also observed at different levels. Without major exhaust sources, ozone horizontal variation has a strong correlation with the vertical convection intensity of air masses within the lower troposphere. Higher air temperatures are usually related to lower ozone horizontal variations at the localized area, whereas underlying surface diversity has a week influence. Three-dimensional ozone maps are obtained using an interpolation method based on UAV collected samples, which are capable of clearly demonstrating the diurnal evolution processes of ozone within the 1000 m lower troposphere.
Show more [+] Less [-]Gas–particle phase partitioning and particle size distribution of chlorinated and brominated polycyclic aromatic hydrocarbons in haze
2017
Jin, Rong | Zheng, Minghui | Yang, Hongbo | Yang, Lili | Wu, Xiaolin | Xu, Yang | Liu, Guorui
Chlorinated and brominated polycyclic aromatic hydrocarbons (Cl/Br-PAHs) are emerging semi-volatile organic pollutants in haze-associated particulate matter (PM). Their gas–particle phase partitioning and distribution among PM fractions have not been clarified. Clarification would increase understanding of atmospheric behavior and health risks of Cl/Br-PAHs. In this study, samples of the gas phase and 4 PM phases (aerodynamic diameters (dae) > 10 μm, 2.5–10 μm, 1.0–2.5 μm, and <1.0 μm) were collected simultaneously during haze events in Beijing and analyzed. Normalized histogram distribution indicated that the Cl/Br-PAHs tended to adhere to fine particles. Over 80% of the Cl-PAHs and 70% of the Br-PAHs were associated with fine PM (dae < 2.5 μm). The gas–particle phase partitioning and PM distribution of Cl/Br-PAHs when heating of buildings was required, which was associated with haze events, were obviously different from those when heating was not required. The relationship between the logarithmic geometric mean diameters of the Cl/Br-PAH congeners and reciprocal of the temperature (1/T) suggested that low air temperatures during the heating period could lead to high proportions of Cl/Br-PAHs in the fine particles. Increased coal burning during the heating period also contributed to high Cl/Br-PAH loads in the fine particles.
Show more [+] Less [-]Hourly associations between heat and ambulance calls
2017
Guo, Yuming
The response speed of ambulance calls is very crucial to rescue patients suffering immediately life threatening conditions. The serious health outcomes might be caused by exposing to extreme heat only several hours before. However, limited evidence is available on this topic. This study aims to examine the hourly association between heat and ambulance calls, to improve the ambulance services and to better protect health.Hourly data on ambulance calls for non-accidental causes, temperature and air pollutants (PM10, NO2, and O3) were collected from Brisbane, Australia, during 2001 and 2007. A time-stratified case-crossover design was used to examine the associations between hourly ambulance calls and temperature during warm season (Nov, Dec, Jan, Feb, and Mar), while adjusting for potential confounders. Stratified analyses were performed for sex and age groups.Ambulance calls peaked at 10am for all groups, except those aged <15 years at 19pm, while temperature was hottest at 13pm. The hourly heat-ambulance calls relationships were non-linear for all groups, with thresholds between 27 °C and 31 °C. The associations appeared immediately, and lasted for about 24 h. There were no significant modification effect by sex and age.The findings suggest that hot hourly temperatures (>27 °C) increase the demands of ambulance. This information is helpful to increase the efficiency of ambulance service then save lives, for example, preparing more ambulance before appearance of extremely hot temperature in combination with weather forecast. Also, people should better arrange their time for outdoor activities to avoid exposing to extreme hot temperatures.
Show more [+] Less [-]Future heat waves due to climate change threaten the survival of Posidonia oceanica seedlings
2017
Guerrero-Meseguer, Laura | Marín, Arnaldo | Sanz-Lázaro, Carlos
Extreme weather events are major drivers of ecological change, and their occurrence is likely to increase due to climate change. The transient increases in atmospheric temperatures are leading to a greater occurrence of heat waves, extreme events that can produce a substantial warming of water, especially in enclosed basins such as the Mediterranean Sea. Here, we tested the effects of current and predicted heat waves on the early stages of development of the seagrass Posidonia oceanica. Temperatures above 27 °C limited the growth of the plant by inhibiting its photosynthetic system. It suffered a reduction in leaf growth and faster leaf senescence, and in some cases mortality. This study demonstrates that the greater frequency of heat waves, along with anticipated temperature rises in coming decades, are expected to negatively affect the germination of P. oceanica seedlings.
Show more [+] Less [-]Impacts of climate and management on water balance and nitrogen leaching from montane grassland soils of S-Germany
2017
Fu, Jin | Gasche, R. | Wang, Na | Lü, Haiyan | Butterbach-Bahl, Klaus | Kiese, Ralf
In this study water balance components as well as nitrogen and dissolved organic carbon leaching were quantified by means of large weighable grassland lysimeters at three sites (860, 770 and 600 m a.s.l.) for both intensive and extensive management. Our results show that at E600, the site with highest air temperature (8.6 °C) and lowest precipitation (981.9 mm), evapotranspiration losses were 100.7 mm higher as at the site (E860) with lowest mean annual air temperature (6.5 °C) and highest precipitation (1359.3 mm). Seepage water formation was substantially lower at E600 (−440.9 mm) as compared to E860. Compared to climate, impacts of management on water balance components were negligible. However, intensive management significantly increased total nitrogen leaching rates across sites as compared to extensive management from 2.6 kg N ha−1 year−1 (range: 0.5–6.0 kg N ha−1 year−1) to 4.8 kg N ha−1 year−1 (range: 0.9–12.9 kg N ha−1 year−1). N leaching losses were dominated by nitrate (64.7%) and less by ammonium (14.6%) and DON (20.7%). The low rates of N leaching (0.8–6.9% of total applied N) suggest a highly efficient nitrogen uptake by plants as measured by plant total N content at harvest. Moreover, plant uptake was often exceeding slurry application rates, suggesting further supply of N due to soil organic matter decomposition. The low risk of nitrate losses via leaching and surface runoff of cut grassland on non-sandy soils with vigorous grass growth may call for a careful site and region specific re-evaluation of fixed limits of N fertilization rates as defined by e.g. the German Fertilizer Ordinance following requirements set by the European Water Framework and Nitrates Directive.
Show more [+] Less [-]Influence of climate change on the multi-generation toxicity to Enchytraeus crypticus of soils polluted by metal/metalloid mining wastes
2017
Barmentlo, S Henrik | van Gestel, Cornelis A.M. | Álvarez-Rogel, José | González-Alcaraz, M Nazaret
This study aimed at assessing the effects of increased air temperature and reduced soil moisture content on the multi-generation toxicity of a soil polluted by metal/metalloid mining wastes. Enchytraeus crypticus was exposed to dilution series of the polluted soil in Lufa 2.2 soil under different combinations of air temperature (20 °C and 25 °C) and soil moisture content (50% and 30% of the soil water holding capacity, WHC) over three generations standardized on physiological time. Generation time was shorter with increasing air temperature and/or soil moisture content. Adult survival was only affected at 30% WHC (∼30% reduction at the highest percentages of polluted soil). Reproduction decreased with increasing percentage of polluted soil in a dose-related manner and over generations. Toxicity increased at 30% WHC (>50% reduction in EC50 in F0 and F1 generations) and over generations in the treatments at 20 °C (40–60% reduction in EC50 in F2 generation). At 25 °C, toxicity did not change when combined with 30% WHC and only slightly increased with 50% WHC. So, higher air temperature and/or reduced soil moisture content does affect the toxicity of soils polluted by metal/metalloid mining wastes to E. crypticus and this effect may exacerbate over generations.
Show more [+] Less [-]Ecological impacts of atmospheric pollution and interactions with climate change in terrestrial ecosystems of the Mediterranean Basin: Current research and future directions
2017
Ochoa-Hueso, Raúl | Munzi, Silvana | Alonso, Rocío | Arróniz-Crespo, María | Avila, Anna | Bermejo, Victoria | Bobbink, Roland | Branquinho, Cristina | Concostrina Zubiri, Laura | Cruz Mínguez, Cristina | Cruz de Carvalho, Ricardo | De Marco, Alessandra | Dias, Teresa | Elustondo, David | Elvira, Susana | Estébanez, Belén | Fusaro, Lina | Gerosa, Giacomo | Izquieta-Rojano, Sheila | Lo Cascio, Mauro | Marzuoli, Riccardo | Matos, Paula | Mereu, Simone | Merino, José | Morillas, Lourdes | Nunes, Alice | Paoletti, Elena | Paoli, Luca | Pinho, Pedro | Rogers, Isabel B. | Santos, Arthur | Sicard, Pierre | Stevens, Carly J. | Theobald, Mark R.
Mediterranean Basin ecosystems, their unique biodiversity, and the key services they provide are currently at risk due to air pollution and climate change, yet only a limited number of isolated and geographically-restricted studies have addressed this topic, often with contrasting results. Particularities of air pollution in this region include high O3 levels due to high air temperatures and solar radiation, the stability of air masses, and dominance of dry over wet nitrogen deposition. Moreover, the unique abiotic and biotic factors (e.g., climate, vegetation type, relevance of Saharan dust inputs) modulating the response of Mediterranean ecosystems at various spatiotemporal scales make it difficult to understand, and thus predict, the consequences of human activities that cause air pollution in the Mediterranean Basin. Therefore, there is an urgent need to implement coordinated research and experimental platforms along with wider environmental monitoring networks in the region. In particular, a robust deposition monitoring network in conjunction with modelling estimates is crucial, possibly including a set of common biomonitors (ideally cryptogams, an important component of the Mediterranean vegetation), to help refine pollutant deposition maps. Additionally, increased attention must be paid to functional diversity measures in future air pollution and climate change studies to establish the necessary link between biodiversity and the provision of ecosystem services in Mediterranean ecosystems. Through a coordinated effort, the Mediterranean scientific community can fill the above-mentioned gaps and reach a greater understanding of the mechanisms underlying the combined effects of air pollution and climate change in the Mediterranean Basin.
Show more [+] Less [-]Particle dry deposition of polycyclic aromatic hydrocarbons and its risk assessment in a typical coal-polluted and basin city, northern China
2017
He, Qiusheng | Zhang, Lu | Cui, Yang | Cheng, Mingchao | Guo, Lili | Liu, Ming | Chen, Laiguo
Atmospheric dry deposition is a major pathway of pollutants removal from the atmosphere to the water and soil ecosystem. Polycyclic aromatic hydrocarbons (PAHs) in Taiyuan, China, are one class of the most hazardous air pollutants due to the high emission intensity from coal consumption. To better understand the PAHs removing from the atmosphere, 16 USEPA priority PAHs (except for naphthalene) in the particle dry deposition samples were detected from August 2013 to November 2014 at an urban site in Taiyuan. Dry deposition fluxes of particles were estimated as 157.44–358.17 mg/(m2·d), with the highest value in spring and lowest in autumn. Particle dry deposition fluxes of ∑15-PAHs ranged from 2436.20 to 14,967.36 ng/(m2·d), and was the highest in winter and lowest in summer. Higher PAHs particle dry deposition fluxes were related to higher PAHs emission, lower air temperature, less precipitation as well as wind speed. Overall dry deposition velocities of 15-PAHs were 0.056 ± 0.027 cm/s in winter and 0.42 ± 0.050 cm/s in summer, respectively, and high molecular weight PAHs showed low dry deposition velocities. Positive matrix factorization model's results indicated that coking, vehicle exhaust, coal combustion were the primary PAHs sources in particle dry deposition samples, accounting for 18.64%, 26.54% and 54.82% of total PAHs, respectively. The toxic equivalent concentrations (BaPeq) of ∑15-PAHs in particle dry deposition samples was in the range of 0.69–2.94 μg/g, which might be a good explanation to high soil PAHs concentrations reported in Shanxi province, China. Furthermore, this work could prove the significance of coal combustion, and related pollution control works are needed to conduct to alleviate the PAHs pollution situation.
Show more [+] Less [-]Ultrafine particles in inhabited areas in the Arctic - From very low to high concentrations
2017
Pétursdóttir, Una | Kirkelund, Gunvor Marie | Press-Kristensen, Kåre | Hertel, Ole | Mikkelsen, Teis Nørgaard
The Arctic is considered a pristine environment, where pollution mainly originates from global sources. The present study examines particle number concentrations (PNCs) and the main sources of airborne ultrafine particles (UFPs, d < 100 nm) in the town Sisimiut and two nearby settlements, Sarfannguit and Itilleq, in West Greenland. Measurements were carried out during three weeks in April and May 2016. Air temperatures during the measurements ranged from −4.4 to +8.7 °C. A portable condensation particle counter (P-Trak) was used for the measurements. Results showed that the lowest concentrations were found during days with high wind speeds, with the lowest PNC average of 72 ± 11 cm−3 (n = 9) (12 m/s). Background concentrations were usually low compared to more densely populated countries, with a couple of exceptions, where there was no clear cause for elevated PNCs in a background area East of Sisimiut. Measured PNCs in the flue gas in the waste incineration plant in Sisimiut showed up to 334,976 cm−3 and are expected to be higher in the gas after it is released through the chimney. Average PNCs up to 77,009 ± 43,880 cm−3 (n = 26) were measured by a road located by the harbor in Sisimiut, while subsequent measurements at the same location showed much lower PNCs. The presence of heavy machinery elevated PNCs highly during two measurement events, giving PNCs up to 270,993 cm−3 but dropping to 1180 cm−3 10 min later, after the vehicle had passed by. A measurement event in Sisimiut Airport while an aircraft landed and departed showed an average PNC of 44,741 ± 85,094 cm−3 (n = 21). Two 24-h measurements resulted in average PNCs of 2960 ± 5704 cm−3 and 3935 ± 10,016 cm−3 respectively.
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