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Occurrence and transport of 17 perfluoroalkyl acids in 12 coastal rivers in south Bohai coastal region of China with concentrated fluoropolymer facilities
2014
Wang, Pei | Lü, Yonglong | Wang, Tieyu | Fu, Yaning | Zhu, Zhaoyun | Liu, Shijie | Xie, Shuangwei | Xiao, Yang | Giesy, John P.
Perfluoroalkyl acids (PFAAs) are emerging contaminants that have raised great concern in recent years. While PFAAs manufacturing becomes regulated in developed countries, production has been partly shifted to China. Eight fluoropolymer manufacturing facilities located in the South Bohai coastal region, one of the most populated areas of China, have been used to manufacture PFAA-related substances since 2001. The environmental consequence of the intensive production of PFAAs in this region remains largely unknown. We analyzed 17 PFAAs in twelve coastal rivers of this region, and found staggeringly high concentrations of perfluorooctanoic acid (PFOA) ranging from 0.96 to 4534.41 ng/L. The highest concentration was observed in the Xiaoqing River which received effluents from certain fluoropolymer facilities. Principal component analysis indicated similar sources of several perfluoroalkyl carboxylic acids (PFCAs) in all rivers, which indicated that atmospheric transport, wastewater treatment and surface runoff also acted as important supplements to direct discharge to surface water.
Show more [+] Less [-]Verification of NOx emission inventories over North Korea
2014
Kim, Na Kyung | Kim, Yong Pyo | Morino, Yu | Kurokawa, Jun-ichi | Ōhara, Toshimasa
In this study, the top-down NOx emissions estimated from satellite observations of NO2 vertical column densities over North Korea from 1996 to 2009 were analyzed. Also, a bottom-up NOx emission inventory from REAS 1.1 from 1980 to 2005 was analyzed with several statistics. REAS 1.1 was in good agreement with the top-down approach for both trend and amount. The characteristics of NOx emissions in North Korea were quite different from other developed countries including South Korea. In North Korea, emissions from industry sector was the highest followed by transportation sector in the 1980s. However, after 1990, the NOx emissions from other sector, mainly agriculture, became the 2nd highest. Also, no emission centers such as urban areas or industrial areas were distinctively observed. Finally, the monthly NOx emissions were high during the warm season.
Show more [+] Less [-]The past and future of fish consumption: Can supplies meet healthy eating recommendations?
2014
Thurstan, Ruth H. | Roberts, Callum M.
In many developed countries fish and shellfish are increasingly promoted as healthy alternatives to other animal protein. We analysed how much fish was available to UK and global populations after accounting for processing losses, and compared this to recommended levels of fish consumption. In 2012, UK domestic fish landings per capita fell 81% below the recommended intake, although declines were masked by increased imports and aquaculture from the 1970s onwards. Global wild fish supply per capita declined by 32% from its peak in 1970. However, overall fish supplies per capita increased by 10% over the same period due to rapidly expanding aquaculture production. Whilst aquaculture has so far prevented a downturn in global fish supplies, many developed nations continue to aspire to consume more fish than they produce. Until demand is balanced with sustainable methods of production governments should consider carefully the social and environmental implications of greater fish consumption.
Show more [+] Less [-]Characterization of fine particulate black carbon in Guangzhou, a megacity of South China
2014
Chen, Xiaocui | Zhang, Zhisheng | Engling, Guenter | Zhang, Renjian | Tao, Jun | Lin, Mang | Sang, Xuefang | Chan, Chuenyu | Li, Shiyu | Li, Youping
Continuous measurement of fine particulate black carbon (BC) was conducted at an urban site of Guangzhou in South China from December 2007 to December 2008. The daily average BC concentrations ranged from 0.6 to 20.5μg m−3, with an average value of 4.7μg m−3, which was substantially higher than those observed in the urban areas of other developed countries. Diurnal fluctuations of BC were marked with two peaks, one in the morning rush hour (08:00LT) and the other in the late evening hour (21:00–22:00LT), while the lowest BC concentrations were observed in the afternoon. Ambient BC concentrations displayed significant seasonal and diurnal variations with higher values in winter and spring, followed by lower concentrations during autumn and summer. Wind speed, wind direction and temperature were important meteorological factors that affected BC concentrations. A clearly negative correlation (r=−0.50, p<0.01) between BC concentrations and wind speed was found during the study period. A specific investigation was conducted to determine the relationship between optical BC and thermal–optical–reflectance elemental carbon (TOR EC) in distinct seasons. Although significant correlations between BC and EC were obtained (r>0.92, p<0.01), the regression slopes (ΔBC/ΔEC) slightly deviated from each other with values of 0.79, 1.18, and 0.81 in winter, spring and summer, respectively, possibly due to the distinct mixing states and source variations in different seasons. The calculated experimental attenuation coefficient showed a higher value (19.3m2g−1) in Guangzhou than the one recommended for typical Aethalometer measurements.
Show more [+] Less [-]Changes in the nature of dissolved organics during pulp and paper mill wastewater treatment: a multivariate statistical study combining data from three analytical techniques
2014
Plant, Emma L. | Smernik, Ronald J. | Leeuwen, John van | Greenwood, Paul | Macdonald, Lynne M.
The paper-making process can produce large amounts of wastewater (WW) with high particulate and dissolved organic loads. Generally, in developed countries, stringent international regulations for environmental protection require pulp and paper mill WW to be treated to reduce the organic load prior to discharge into the receiving environment. This can be achieved by primary and secondary treatments involving both chemical and biological processes. These processes result in complex changes in the nature of the organic material, as some components are mineralised and others are transformed. In this study, changes in the nature of organics through different stages of secondary treatment of pulp and paper mill WW were followed using three advanced characterisation techniques: solid-state¹³C nuclear magnetic resonance (NMR) spectroscopy, pyrolysis-gas chromatography mass spectrometry (py-GCMS) and high-performance size-exclusion chromatography (HPSEC). Each technique provided a different perspective on the changes that occurred. To compare the different chemical perspectives in terms of the degree of similarity/difference between samples, we employed non-metric multidimensional scaling. Results indicate that NMR and HPSEC provided strongly correlated perspectives, with 86 % of the discrimination between the organic samples common to both techniques. Conversely, py-GCMS was found to provide a unique, and thus complementary, perspective.
Show more [+] Less [-]The potential of the flora from different regions of Pakistan in phytoremediation: a review
2014
Kamran, Muhammad Aqeel | Amna, | Mufti, Rabia | Mubariz, Nadia | Syed, Jabir Hussain | Bano, Asghari | Javed, Muhammad Tariq | Munis, Muhammad Farooq Hussain | Tan, Zhiyuan | Chaudhary, Hassan Javed
Soil and water quality is greatly affected by environmental pollution due to the increasing trend of urbanization and industrialization. In many developing countries, including Pakistan, the situation is more alarming as no preventive measures are still taken to tackle the problem. Although in developed countries, many techniques are used to remediate the environment including phytoremediation. It is the most eco-friendly technique in which plants are used to remove pollutants from the environment. Pakistan has also a great diversity of plants which could be used for the remediation of environmental pollutants. To our knowledge, few studies from Pakistan were reported about the use of flora for phytoremediation. According to recent literature, 50 plant species from Pakistan are studied for remediation purposes. In this review, the potential of different plant species for phytoremediation from Pakistan has been discussed along with their comparison to other countries to relate future perspectives.
Show more [+] Less [-]Development of aquatic life criteria in China: viewpoint on the challenge
2014
Jin, Xiaowei | Wang, Yeyao | Giesy, John P. | Richardson, Kristine L. | Wang, Zijian
While more developed countries have a well-established systems to develop water quality criteria (WQC), little research has been done on the adequacy of the current WQC to protect endemic species of China. In order to maintain the health of aquatic ecosystems in China, a series of projects to establish national WQC based on regional characteristics has recently been initiated. However, the establishment of a completely novel methodology would be costly and time consuming. Also, due to the similarities in physiologies and natural histories of classes of aquatic organisms, there is no reason to believe that WQC would not be sufficient to protect unique species in China. This review was undertaken to identify key outstanding issues regarding establishment of aquatic life criteria (ALC) to be applied in China, including prioritization of chemicals, test species, mode of action, field/semi-field data, and methods of aggregating the information and calculating the ALC. This was used to identify the principle issues that need to be addressed in order to better understand the methods for development of criteria for the protection of aquatic life and provide a reference to China and other developing countries committed to the establishment of their own WQC system.
Show more [+] Less [-]Development and implementation of surface water quality standards for protection of human health in Korea
2014
An, Youn-Joo | Kwak, Jin II | Nam, Sun-Hwa | Jung, Myung-sook
Current water quality standards for the protection of human health in Korea include 17 substances found in rivers and streams. Due to increasing concern over the release of hazardous chemicals into the aquatic environment, there has been a demand for additional water quality standards. Therefore, the Korean Ministry of the Environment plans to gradually increase the number of water quality standards to 30 substances, including 22 substances for protection of human health and 8 substances for protection of aquatic ecosystems by 2015. In this study, new water quality standards for protection of human health were established for 1,4-dioxane, formaldehyde, and hexachlorobenzene. We selected candidate hazardous chemicals, conducted a human health risk assessment to determine priority chemicals, established water quality standards based on technical analyses and comparison with domestic and developed countries’ water quality standards, and conducted an expert review. Water quality standards for protection of aquatic ecosystems will be derived in the near future. This study describes how the water quality standards for protection of human health were developed and implemented. Current status, recent expansion, and future plans for water quality standards in Korea are also covered.
Show more [+] Less [-]The challenges of reducing greenhouse gas emissions and air pollution through energy sources: evidence from a panel of developed countries
2014
Akhmat, Ghulam | Zaman, Khalid | Shukui, Tan | Sajjad, Faiza | Khan, Muhammad Azhar | Khan, Muhammad Zahir
The objective of the study is to investigate the long-run relationship between climatic factors (i.e., greenhouse gas emissions, agricultural methane emissions, and industrial nitrous oxide emission), air pollution (i.e., carbon dioxide emissions), and energy sources (i.e., nuclear energy; oil, gas, and coal energy; and fossil fuel energy) in the panel of 35 developed countries (including EU-15, new EU member states, G-7, and other countries) over a period of 1975–2012. In order to achieve this objective, the present study uses sophisticated panel econometric techniques including panel cointegration, panel fully modified OLS (FMOLS), and dynamic OLS (DOLS). The results show that there is a long-run relationship between the variables. Nuclear energy reduces greenhouse gases and carbon emissions; however, the other emissions, i.e., agricultural methane emissions and industrial nitrous oxide, are still to increase during the study period. Electricity production from oil, gas, and coal sources increases the greenhouse gases and carbon emissions; however, the intensity to increase emissions is far less than the intensity to increase emissions through fossil fuel. Policies that reduce emissions of greenhouse gases can simultaneously alter emissions of conventional pollutants that have deleterious effects on human health and the environment.
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