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Comparison of the Chemical Composition of Precipitation on the Western and Eastern Coasts of Korea
2004
Kang, Gongunn | Collett, Jeffrey L., Jr | Shin, Dae-Ywen | Fujita Shin'ichi, | Kim, Hui-Kang
Precipitation samples were collected at two coastal sites on the Korean Peninsula, Kangwha on the western coast and Yangyang on the eastern coast, from September 1991 to February 1997. The samples were analyzed for concentrations of major ions, in addition to pH and electrical conductivity. The annual volume-weighted mean pH values were 4.89 and 5.05 at Kangwha and Yangyang, respectively. The pH was generally lower at Kangwha than that at Yangyang, especially during the winter, because of reduced neutralizing inputs and greater acid inputs in winter. Dominant ions were different with NH₄ ⁺ and SO₄ ²⁻ most important at Kangwha and Na⁺ and Cl⁻ at Yangyang. Neglecting sea salt components, nss-SO₄ ²⁻ and NO₃ ⁻ were important anions and nss-Ca²⁺ and NH₄ ⁺ were important cations at both sites. Concentrations of these ions were 1.2–1.6 times higher at Kangwha than at Yangyang. Annual mean concentrations of these ions varied little during the study, while larger seasonal variations were observed. Annual mean nss-SO₄ ²⁻/NO₃ ⁻ ratios at Kangwha and Yangyang were 2.8 and 2.6. The 5 yr annual mean values of nss-SO₄ ²⁻/NO₃ ⁻ showed no trend at Kangwha but a decreasing tendency at Yangyang. The decreasing trend is similar to the decreasing trend in emissions of SO₂/NOₓ in South Korea. Regional differences in chemical composition between Kangwha and Yangyang appear to be associated with long-range transport of acidic gases and alkaline dust originated from other regions.
Show more [+] Less [-]Trend and Variability of Total Gaseous Mercury (TGM) in the State of Connecticut, U.S.A. during 1997–1999
2004
Chen, Hao | Yang, Xiusheng | Perkins, Christopher
A statewide total gaseous mercury (TGM) monitoring campaign was conducted from January 1997 to December 1999 in the State of Connecticut, U.S.A. Eight monitoring sites with different characteristics of geographical location (coastal vs. interior) and land use (rural vs. urban) were included in the monitoring program. Statistical procedures were utilized to evaluate the temporal trend and spatial distribution of the TGM concentration in the State, and the influence of long-range transport from non-local sources. The statewide mean TGM concentration was 2.08 ng m⁻³. The annual mean concentration had no significant differences among the three years of measurements for all the sites. Weak seasonal variations were detected in the State with higher ambient TGM concentration found in warmer seasons. Urban areas in general had higher TGM concentrations than rural areas. The effect of site location of the monitoring sites on TGM concentration was interacted with land use characteristics. Waterbury site with extremely high concentration measurements was the major cause for this interaction. The long-range transport of TGM from remote sources showed an important influence on local ambient concentrations, by explaining over 45% of the total variance of the ambient TGM concentration for most sites. Local sources were responsible for the extremely high TGM concentration in the Waterbury site. The TGM concentrations at Voluntown, Hammonasset and Avery Point in southeast Connecticut were likely to be affected by some local sources.
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