Rhodium-Catalyzed Directed C–H Cyanation of Arenes with N-Cyano-N-phenyl-p-toluenesulfonamide
2013
Gong, Tian-Jun | Xiao, Bin | Cheng, Wan-Min | Su, Wei | Xu, Jun | Liu, Zhao-Jing | Liu, Lei | Fu, Yao
A Rh-catalyzed directed C–H cyanation reaction was developed for the first time as a practical method for the synthesis of aromatic nitriles. N-Cyano-N-phenyl-p-toluenesulfonamide, a user-friendly cyanation reagent, was used in the transformation. Many different directing groups can be used in this C–H cyanation process, and the reaction tolerates a variety of synthetically important functional groups.
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