Source apportionment, ecological, and human health risks of toxic metals in road dust of densely populated capital and connected major highway of Bangladesh

Haque, Md Morshedul; Sultana, Sajin; Niloy, Nahin Mostofa; Quraishi, Shamshad B.; Tareq, Shafi M.

Source apportionment, ecological, and human health risks of toxic metals in road dust of densely populated capital and connected major highway of Bangladesh

2022

Haque, Md Morshedul | Sultana, Sajin | Niloy, Nahin Mostofa | Quraishi, Shamshad B. | Tareq, Shafi M.

This study investigates pollution levels, source apportionment, ecological, and human health risks associated with toxic metals (Pb, As, Hg, Cr, and Cd) in road dust from the most populated Dhaka city and a connected major highway in Bangladesh. The mean concentration of Pb, Hg, and Cd were 1.3, 29.3, and 13.2 times higher than their corresponding background values with spatially uneven distribution all over the study area. Metal pollution indices, the geo-accumulation index (Igₑₒ), NIPI, and PI, indicated extreme contamination at many sites depending on local environmental factors. The potential ecological risk ([Formula: see text] revealed that 84% and 54% of samples showed the extreme ecological risk for Hg and Cd pollution, respectively. On the other hand, the potential ecological risk index (PERI) and Nemerow integrated risk index (NIRI) showed that most sampling sites suffered high to extreme ecological risk. Source apportionment using positive matrix factorization (PMF) identified coal combustion, and gasoline (50.14%), traffic exhaust (35.26%), and industrial and agriculture activity (14.60%) were the main source of toxic metals of the study area. Non-carcinogenic health risk indicated that adults are more vulnerable than children, and hazard index (HI) of Hg for both age groups and Cd for adults were significantly higher than the safe level. The carcinogenic risk (CR) levels of toxic metals were acceptable (10⁻⁶ to 10⁻⁴), although the maximum limit of Cr for children and As for adults was close to the unacceptable limit (10⁻⁴). Continual exposure to toxic metals through road dust might develop lifetime cancer risk in local inhabitants.

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