Measurement of ²²⁴Ra:²²⁸Th disequilibrium in coastal sediments using a delayed coincidence counter
2012
Cai, Pinghe | Shi, Xiangming | Moore, Willard S. | Dai, Minhan
We describe a method for measuring ²²⁴Ra and ²²⁸Th activities in coastal sediments based on a delayed-coincidence counting system (the RaDeCC system). Milli-Q water is added to bulk sediment to form a slurry. ²²⁴Ra in interstitial water is co-precipitated by MnO₂ suspension. The MnO₂ suspension and the sediment with absorbed ²²⁴Ra and ²²⁸Th are filtered onto a 142-mm 0.7μm (nominal pore size) GFF filter. The filter is placed onto a sample holder specified for sediment samples and counted in a RaDeCC system. ²²⁴Ra and ²²⁸Th activities are calculated from two measurements that are conducted within 6–12h and in 8–10days after sample collection. The RaDeCC system is calibrated with a ²³²U-²²⁸Th standard using the method of standard addition. The reproducibility and the overall accuracy of ²²⁴Ra and ²²⁸Th measurements based on this method are estimated to be ±5% and ±5–7%, respectively. We have applied this method to a coastal sediment and observed a significant deficit of ²²⁴Ra with respect to ²²⁸Th in the upper 3–4cm.
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