Enhanced quantum yield of nitrogen fixation for hydrogen storage with in situ-formed carbonaceous radicals
2015
Zhao, Weirong | Xi, Haiping | Zhang, Meng | Li, Yajun | Chen, Jinsheng | Zhang, Jing | Zhu, Xi
NH₃ is a potential hydrogen energy carrier. Here we use alcohols as hole scavengers to investigate the nitrogen photofixation mechanisms including direct and indirect electron transfer processes. The t-butanol system exhibited the highest quantum yield of 36.1%, ascribing to the in situ-formed indirect electronic transmitter ˙CO₂⁻.
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