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Road Traffic and PM10, PM2.5 Emission at an Urban Area in Algeria: Identification and Statistical Analysis Texte intégral
2020
Belarbi, N. | Belamri, M. | Dahmani, B. | Benamar, M. A.
Air quality in greater Algiers, in Algeria was assessed analyzing aerosol particulate matter (PM10 and PM2.5) at a site influenced by heavy road traffic. Particulate matters were collected using a Gent sampler to characterize the atmospheric aerosol of Algiers. An Energy dispersive X ray spectrometer (EDXRF) was used to determine the heavy metal concentrations in the PM2.5 and PM10 size fractions. Principal Component analysis and Enrichment factor were used to identify the major sources of air pollutants for PM10 fraction in the studied area. Backward trajectories were calculated in order to identify potential distant sources that contribute to particulate pollution in our site. Significant concentrations of PM 2.5 and PM10 as well as associated heavy metals have been documented. The mean concentrations of heavy metals contained in PM10 and PM2.5 were, in descending order, Fe>Zn>Ni>Pb>Mn>Co>Cr; Pb>Mn>Co>Fe>Zn>Ni>Cr respectively. The contribution of road traffic to the levels of fine (PM2.5), and coarse (PM10) particles were studied.
Afficher plus [+] Moins [-]Metal Signature of Atmospheric Aerosol from Kochi, the Queen of Arabian Sea, Kerala, India Texte intégral
2016
K, Gayathree Devi | P.S., Akhil | C.H., Sujatha
The present research article highlights the metal (Cd, Cu, Pb, Zn and Fe)distribution pattern in the RSPM generated in different hot spot sites located at Kochi, theQueen of Arabian Sea. These sampling sites are categorized under three different zonesas estuarine, riverine, and coastal. Two sampling phases are selected in order to check theconsistency in pollution trend after a two year gap and are described in Phase I and PhaseII, respectively. Metals are noticed to be intensely concentrated in the post monsoonmonths in both phases. Among the metals, Fe is revealed as the prominent metal at theestuarine sites. Estuarine and riverine zone expresses the overall enrichment pattern withslight difference at coastal regime in phase I. In phase II, insignificant metal load withirregular pattern is observed. Source apportionment study reveals that major sources ofmetals are from automobile exhausts and the estuarine zone is entangled with 45.9%.
Afficher plus [+] Moins [-]Changement du systeme climatique: les dernieres decouvertes scientifiques.
1994
Acidity of size-fractionated aerosol particles.
1990
Ludwig J. | Klemm O.
Diurnal variations of aerosol concentrations inside and above a young spruce stand: modelling and measurements.
1986
Wiman B.L.B.
Carbonaceous aerosol at urban and rural sites in the United States.
1986
Shah J.J. | Johnson R.L. | Heyerdahl E.K. | Huntzicker J.J.
The feedback effects of aerosols from different sources on the urban boundary layer in Beijing China Texte intégral
2023
Xin, Jinyuan | Ma, Yongjing | Zhao, Dandan | Gong, Chongshui | Ren, Xinbing | Tang, Guiqian | Xia, Xiangao | Wang, Zifa | Cao, Junji | de Arellano, Jordi Vilà Guerau | Martin, Scot T.
The interaction of aerosols and the planetary boundary layer (PBL) plays an important role in deteriorating urban air quality. Aerosols from different sources may have different effects on regulating PBL structures owing to their distinctive dominant compositions and vertical distributions. To characterize the complex feedback of aerosols on PBL over the Beijing megacity, multiple approaches, including in situ observations in the autumn and winter of 2016–2019, backward trajectory clusters, and large-eddy simulations, were adopted. The results revealed notable distinctions in aerosol properties, vertical distributions and thermal stratifications among three types of air masses from the West Siberian Plain (Type-1), Central Siberian Plateau (Type-2) and Mongolian Plateau (Type-3). Low loadings of 0.28 ± 0.26 and 0.15 ± 0.08 of aerosol optical depth (AOD) appeared in the Type-1 and Type-2, accompanied by cool and less stable stratification, with a large part (80%) of aerosols concentrated below 1500 m. For Type-3, the AOD and single scattering albedo (SSA) were as high as 0.75 ± 0.54 and 0.91 ± 0.05, demonstrating severe pollution levels of abundant scattering aerosols. Eighty percent of the aerosols were constrained within a lower height of 1150 m owing to the warmer and more stable environment. Large-eddy simulations revealed that aerosols consistently suppressed the daytime convective boundary layer regardless of their origins, with the PBL height (PBLH) decreasing from 1120 m (Type-1), 1160 m (Type-2) and 820 m (Type-3) in the ideal clean scenarios to 980 m, 1100 m and 600 m, respectively, under polluted conditions. Therefore, the promotion of absorbing aerosols below the residual layer on PBL could be greatly hindered by the suppression effects generated by both absorbing aerosols in the upper temperature inversion layer and scattering aerosols. Moreover, the results indicated the possible complexities of aerosol-PBL interactions under future emission-reduction scenarios and in other urban regions.
Afficher plus [+] Moins [-]Vertical profiles of the transport fluxes of aerosol and its precursors between Beijing and its southwest cities Texte intégral
2022
Hu, Qihou | Liu, Cheng | Li, Qihua | Liu, Ting | Ji, Xiangguang | Zhu, Yizhi | Xing, Chengzhi | Liu, Haoran | Tan, Wei | Gao, Meng
The influence of regional transport on aerosol pollution has been explored in previous studies based on numerical simulation or surface observation. Nevertheless, owing to inhomogeneous vertical distribution of air pollutants, vertical observations should be conducted for a comprehensive understanding of regional transport. Here we obtained the vertical profiles of aerosol and its precursors using ground-based multi-axis differential optical absorption spectroscopy (MAX-DOAS) at the Nancheng site in suburban Beijing on the southwest transport pathway of the Beijing-Tianjin-Hebei (BTH) region, China, and then estimated the vertical profiles of transport fluxes in the southwest-northeast direction. The maximum net transport fluxes per unit cross-sectional area, calculated as pollutant concentration multiply by wind speed, of aerosol extinction coefficient (AEC), NO₂, SO₂ and HCHO were 0.98 km⁻¹ m s⁻¹, 24, 14 and 8.0 μg m⁻² s⁻¹ from southwest to northeast, which occurred in the 200–300 m, 100–200 m, 500–600 m and 500–600 m layers, respectively, due to much higher pollutant concentrations during southwest transport than during northeast transport in these layers. The average net column transport fluxes were 1200 km⁻¹ m² s⁻¹, 38, 26 and 15 mg m⁻¹ s⁻¹ from southwest to northeast for AEC, NO₂, SO₂ and HCHO, respectively, in which the fluxes in the surface layer (0–100 m) accounted for only 2.3%–4.2%. Evaluation only based on surface observation would underestimate the influence of the transport from southwest cities to Beijing. Northeast or weak southwest transports dominated in clean conditions with PM₂.₅ <75 μg m⁻³ and intense southwest transport dominated in polluted conditions with PM₂.₅ >75 μg m⁻³. Southwest transport through the middle boundary layer was a trigger factor for aerosol pollution events in urban Beijing, because it not only directly bringing air pollutants, but also induced an inverse structure of aerosols, which resulted in stronger atmospheric stability and aggravated air pollution in urban Beijing.
Afficher plus [+] Moins [-]Vertical profile of aerosols in the Himalayas revealed by lidar: New insights into their seasonal/diurnal patterns, sources, and transport Texte intégral
2021
Xiang, Yan | Zhang, Tianshu | Liu, Jianguo | Wan, Xin | Loewen, Mark | Chen, Xintong | Kang, Shichang | Fu, Yibin | Lv, Lihui | Liu, Wenqing | Cong, Zhiyuan
Atmospheric aerosols play a crucial role in climate change, especially in the Himalayas and Tibetan Plateau. Here, we present the seasonal and diurnal characteristics of aerosol vertical profiles measured using a Mie lidar, along with surface black carbon (BC) measurements, at Mt. Qomolangma (QOMS), in the central Himalayas, in 2018–2019. Lidar-retrieved profiles of aerosols showed a distinct seasonal pattern of aerosol loading (aerosol extinction coefficient, AEC), with a maximum in the pre-monsoon (19.8 ± 22.7 Mm⁻¹ of AEC) and minimum in the summer monsoon (7.0 ± 11.2 Mm⁻¹ of AEC) seasons. The diurnal variation characteristics of AEC and BC were quite different in the non-monsoon seasons with enriched aerosols being maintained from 00:00 to 10:00 in the pre-monsoon season. The major aerosol types at QOMS were identified as background, pollution, and dust aerosols, especially during the pre-monsoon season. The occurrence of pollution events influenced the vertical distribution, seasonal/diurnal patterns, and types of aerosols. Source contribution of BC based on the weather research and forecasting chemical model showed that approximately 64.2% ± 17.0% of BC at the QOMS originated from India and Nepal in South Asia during the non-monsoon seasons, whereas approximately 47.7% was from local emission sources in monsoon season. In particular, the high abundance of BC at the QOMS in the pre-monsoon season was attributed to biomass burning, whereas anthropogenic emissions were the likely sources during the other seasons. The maximum aerosol concentration appeared in the near-surface layer (approximately 4.3 km ASL), and high concentrations of transported aerosols were mainly found at 4.98, 4.58, 4.74, and 4.88 km ASL in the pre-monsoon, monsoon, post-monsoon, and winter seasons, respectively. The investigation of the vertical profiles of aerosols at the QOMS can help verify the representation of aerosols in the air quality model and satellite products and regulate the anthropogenic disturbance over the Tibetan Plateau.
Afficher plus [+] Moins [-]Interactive effects of air pollutants and atmospheric moisture stress on aspen growth and photosynthesis along an urban-rural gradient Texte intégral
2020
Wang, Zhenhua | Wang, Chengzhang | Wang, Bin | Wang, Xin | Li, Jing | Wu, Jin | Liu, Lingli
Atmospheric pollution could significantly alter tree growth independently and synergistically with meteorological conditions. North China offers a natural experiment for studying how plant growth responds to air pollution under different meteorological conditions, where rapid economic growth has led to severe air pollution and climate changes increase drought stress. Using a single aspen clone (Populus euramericana Neva.) as a ‘phytometer’, we conducted three experiments to monitor aspen leaf photosynthesis and stem growth during in situ exposure to atmospheric pollutants along the urban-rural gradient around Beijing. We used stepwise model selection to select the best multiple linear model, and we used binned regression to estimate the effects of air pollutants, atmospheric moisture stress and their interactions on aspen leaf photosynthesis and growth. Our results indicated that ozone (O₃) and vapor pressure deficit (VPD) inhibited leaf photosynthesis and stem growth. The interactive effect of O₃ and VPD resulted in a synergistic response: as the concentration of O₃ increased, the negative impact of VPD on leaf photosynthesis and stem growth became more severe. We also found that nitrogen (N) deposition had a positive effect on stem growth, which may have been caused by an increase in canopy N uptake, although this hypothesis needs to be confirmed by further studies. The positive impact of aerosol loading may be due to diffuse radiation fertilization effects. Given the decline in aerosols and N deposition amidst increases in O₃ concentration and drought risk, the negative effects of atmospheric pollution on tree growth may be aggravated in North China. In addition, the interaction between O₃ and VPD may lead to a further reduction in ecosystem productivity.
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