Integration of an atmospheric dispersion model with a dynamic multimedia fate model: Development and illustration

Morselli, Melissa; Ghirardello, Davide; Semplice, Matteo; Raspa, Giuseppe; Di Guardo, Antonio

Integration of an atmospheric dispersion model with a dynamic multimedia fate model: Development and illustration

2012

Morselli, Melissa | Ghirardello, Davide | Semplice, Matteo | Raspa, Giuseppe | Di Guardo, Antonio

Growing attention is devoted to understand the influence of the short-term variations in air concentrations on the environmental fate of semivolatile organic compounds (SVOCs) such as polycyclic aromatic hydrocarbons (PAHs). These variations are ascribable to factors such as temperature-mediated air-surface exchange and variability of planetary boundary layer (PBL) height and structure. But when investigating the fate of SVOCs at a local scale, further variability can derive from specific point source contributions. In this context, a new modeling approach (AirPlus) which integrates a previously developed model (AirFug) with an air dispersion model (AERMOD) is presented. The integrated model is illustrated for two PAHs in a Northern Italy scenario. Results show how chemical contributions deriving from background advective inflows, local emissions and a point source interact in an hourly-varying meteorological scenario to determine air concentration rapid changes and the consequent response of the soil compartment.

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