Spatiotemporal variability of fugitive gas migration emissions around a petroleum well
2021
Fleming, N.A. | Morais, T.A. | Mayer, K.U. | Ryan, M.C.
Well integrity failure resulting in migration of natural gas outside of the surface casing can cause atmospheric greenhouse gas emissions and groundwater quality impacts from existing and historic energy wells. Spatial and temporal variability in gas migration can result in errors in detection (i.e., presence/absence) and efflux estimations. This field-based case study used automated dynamic closed chambers to record repeated (~every 18 min) CO₂ and CH₄ efflux measurements over a two-week period around a single petroleum production well in Alberta, Canada. Long-term efflux measurements supplemented soil gas compositional and isotopic characterization, along with surface concentration measurements. Effluxes were spatially concentrated around the wellhead and only occasionally detectable more than a few meters away. Estimated total emissions attributable to gas migration ranged from 48 to 466 g CH₄ d⁻¹ (or 0.07–0.7 m³ CH₄ d⁻¹). Methane effluxes and concentrations were temporally variable on second-to-hourly and diel scales. Multivariate stepwise regression analysis indicates that multiple meteorological factors, particularly wind speed and air temperature, were related to the temporal variability. Despite temporal variability, elevated concentrations and effluxes were consistently detectable around the well. Major soil gas composition suggests that gas migration near the wellhead causes advective displacement of soil gas, while more distal measurements are indicative of episodic and diffusion-dominated transport. Values of ¹³C–CO₂ and ¹³C–CH₄ samples were consistent with CH₄ oxidation within the unsaturated zone. Although these results reflect a single well, the findings are salient to gas migration detection and emission estimation efforts.
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