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Artificial radionuclides 90Sr and 241Am in the sediments of the Baltic Sea: Total and spatial inventories and some temporal trends
2013
Hutri, Kaisa-Leena | Mattila, Jukka | Ikäheimonen, Tarja Tuulikki | Vartti, Vesa-Pekka
The Baltic Sea was contaminated by radioactivity following global nuclear fallout and later by the Chernobyl accident. Despite the decrease of radioactivity caused by radioactive decay, radionuclides have a prolonged residence time in the water of the Baltic Sea due to slow water exchange and relatively rapid sedimentation. Very little is known about the amounts or spatial differences of 90Sr and 241Am in the Baltic Sea sediments. In this study, 20 sediment cores taken around the Baltic Sea were investigated to estimate inventories of these radionuclides. The rough results show that the Chernobyl fallout added the amount of 90Sr in the same areas where the increase of 137Cs can be detected, whereas this is not the case for 241Am which is more evenly distributed in the sea bottom. In addition, local differences occur in the concentrations. These results are an important amendment to the radioactivity baseline of the Baltic Sea.
显示更多 [+] 显示较少 [-]Hydrochemical modelling of the retention and transport of metallic radionuclides in the soils of an upland catchment
1996
Tipping, E. (Institute of Freshwater Ecology, Windermere Laboratory, Ambleside, Cumbria LA22 0LP (United Kingdom))
The use of rice and coffee husks for biosorption of U (total), 241Am, and 137Cs in radioactive liquid organic waste
2020
Ferreira, Rafael Vicente de Pádua | de Araujo, Leandro Goulart | Canevesi, Rafael Luan Sehn | da Silva, Edson Antonio | Ferreira, Eduardo Gurzoni Alvares | Palmieri, Maurício Cesar | Marumo, Júlio Takehiro
Rice and coffee husks (raw and chemically activated) are examined as potential biosorption materials regarding their capacity to remove U (total), ²⁴¹Am, and ¹³⁷Cs. The physical parameters evaluated were the morphological characteristics of the biomass, real and apparent density, and surface area. Contact times for the batch experiments were 0.5, 1, 2, and 4 h, and the concentrations tested ranged between 10% of the total concentration and the radioactive waste itself without any dilution. The results were evaluated by experimental sorption capacity, ternary isotherm, and kinetics models. The kinetics results showed that equilibrium was reached after 2 h for all biomass. Raw coffee husk showed the best adsorption results in terms of maximum capacity (qₘₐₓ) for all three radionuclides, which were 1.96, 39.4 × 10⁻⁶, and 46.6 × 10⁻⁹ mg g⁻¹ for U, Am, and Cs, respectively. The biosorption process for the raw and activated rice husks was best represented by the Langmuir ternary isotherm model with two sites. For the coffee husk, in the raw and activated states, the biosorption process was best described by the modified Jain and Snoeyink ternary model. These results suggest that biosorption with these biomaterials can be applied in the treatment of liquid organic radioactive waste containing mainly uranium and americium.
显示更多 [+] 显示较少 [-]Phytoremediation: role of terrestrial plants and aquatic macrophytes in the remediation of radionuclides and heavy metal contaminated soil and water
2015
Sharma, Sunita | Singh, Bikram | Manchanda, V. K.
Nuclear power reactors are operating in 31 countries around the world. Along with reactor operations, activities like mining, fuel fabrication, fuel reprocessing and military operations are the major contributors to the nuclear waste. The presence of a large number of fission products along with multiple oxidation state long-lived radionuclides such as neptunium (²³⁷Np), plutonium (²³⁹Pu), americium (²⁴¹/²⁴³Am) and curium (²⁴⁵Cm) make the waste streams a potential radiological threat to the environment. Commonly high concentrations of cesium (¹³⁷Cs) and strontium (⁹⁰Sr) are found in a nuclear waste. These radionuclides are capable enough to produce potential health threat due to their long half-lives and effortless translocation into the human body. Besides the radionuclides, heavy metal contamination is also a serious issue. Heavy metals occur naturally in the earth crust and in low concentration, are also essential for the metabolism of living beings. Bioaccumulation of these heavy metals causes hazardous effects. These pollutants enter the human body directly via contaminated drinking water or through the food chain. This issue has drawn the attention of scientists throughout the world to device eco-friendly treatments to remediate the soil and water resources. Various physical and chemical treatments are being applied to clean the waste, but these techniques are quite expensive, complicated and comprise various side effects. One of the promising techniques, which has been pursued vigorously to overcome these demerits, is phytoremediation. The process is very effective, eco-friendly, easy and affordable. This technique utilizes the plants and its associated microbes to decontaminate the low and moderately contaminated sites efficiently. Many plant species are successfully used for remediation of contaminated soil and water systems. Remediation of these systems turns into a serious problem due to various anthropogenic activities that have significantly raised the amount of heavy metals and radionuclides in it. Also, these activities are continuously increasing the area of the contaminated sites. In this context, an attempt has been made to review different modes of the phytoremediation and various terrestrial and aquatic plants which are being used to remediate the heavy metals and radionuclide-contaminated soil and aquatic systems. Natural and synthetic enhancers, those hasten the process of metal adsorption/absorption by plants, are also discussed. The article includes 216 references.
显示更多 [+] 显示较少 [-]Sources and distribution of 241Am in the vicinity of a deep geologic repository
2019
Thakur, Punam | Ward, Anderson L.
The detection, distribution, and long-term behavior of ²⁴¹Am in the terrestrial environment at the Waste Isolation Pilot Plant (WIPP) site were assessed using historical data from an independent monitoring program conducted by the Carlsbad Environmental Monitoring & Research Center (CEMRC), and its predecessor organization the Environmental Evaluation Group (EEG). An analysis of historical data indicates frequent detections of trace levels of ²⁴¹Am in the WIPP environment. Positive detections and peaks in ²⁴¹Am concentrations in ambient air samples generally occur during the March to June timeframe, which is when strong and gusty winds in the area frequently give rise to blowing dust. A study of long-term measurements of ²⁴¹Am in the WIPP environment suggest that the resuspension of previously contaminated soils is likely the primary source of americium in the ambient air samples from WIPP and its vicinity. Furthermore, the ²⁴¹Am/²³⁹ ⁺ ²⁴⁰Pu ratio in aerosols and soils was reasonably consistent from year to year and was in agreement with the global fallout ratios. Higher than normal activity concentrations of ²⁴¹Am and ²⁴¹Am/²³⁹ ⁺ ²⁴⁰Pu ratios were measured in aerosol samples during 2014 as a result of February 14, 2014 radiation release event from the WIPP underground. However, after a brief spike, the activity concentrations of ²⁴¹Am have returned to the normal background levels. The long-term monitoring data suggest there is no persistent contamination and no lasting increase in radiological contaminants in the region that can be considered significant by any health-based standard.
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