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Characteristics and health risk assessment of volatile organic compounds (VOCs) in restaurants in Shanghai
2020
Huang, Xiqian | Han, Deming | Cheng Jinping, | Chen, Xiaojia | Zhou, Yong | Liao, Haoxiang | Dong, Wei | Yuan, Chao
Volatile organic compounds (VOCs) are important precursors of ozone and atmospheric particulates that have attracted extensive attention worldwide. Cooking emissions, the chemical characteristics of which vary dramatically due to different cooking styles, are a main source of ambient VOCs, especially in large cities. This research focused on the emission characteristics of VOCs from six types of restaurants in Shanghai: hot pot (HP), Sichuan cuisine (SC), Cantonese cuisine (CS), seafood (SF), Western fast food (WFF), and authentic Shanghai cuisine (ASC). It was found that HP, which discharged cooking fumes indoors, produced the highest mass concentration of VOCs (1900.2 ± 364.8 μg m⁻³), followed by SC (1403.7 ± 403.8 μg m⁻³), WFF (656.0 ± 156.9 μg m⁻³), SF (638.6 ± 145.1 μg m⁻³), CC (632.7 ± 127.7 μg m⁻³), and ASC (612.3 ± 51.3 μg m⁻³), the cooking fumes from which were collected by emission extraction stacks. Additionally, the VOC species from each cuisine were mainly low carbon substances. Alkanes were the major VOC pollutants from all six cuisines, accounting for 34.4–71.7%. The coefficient divergence values were 0.287–0.593, suggesting that there were differences between the cuisines in the present study. Ozone formation potential and secondary organic aerosol formation potential indicated that O-VOCs and aromatics were the largest contributors. Health risk assessment of VOCs via non-carcinogenic risk values (HQ) and carcinogenic risk values (RISK) indicated that frying, grilling, and stir-frying had relatively large impacts on human health. VOCs collected in emission extraction stacks were significantly higher risk compared with those in the indoor environment, but the RISK score of the HP restaurant was larger, second only to SC. The HQ and RISK values of 1,3-butadiene, acetaldehyde, and trichloroethylene in the HP restaurant all exceeded US EPA standards, indicating that long-term exposure in an HP restaurant would have a significant impact on human health and might carry a potential cancer risk.
显示更多 [+] 显示较少 [-]Quantifying trace elements in the emitted particulate matter during cooking and health risk assessment
2017
Gorjinezhad, Soudabeh | Kerimray, Aiymgul | Amouei Torkmahalleh, Mehdi | Keleş, Melek | Ozturk, Fatma | Hopke, Philip K.
Particulate matter (PM) measurements were conducted during heating corn oil, heating corn oil mixed with the table salt and heating low fat ground beef meat using a PTFE-coated aluminum pan on an electric stove with low ventilation. The main objectives of this study were to measure the size segregated mass concentrations, emission rates, and fluxes of 24 trace elements emitted during heating cooking oil or oil with salt and cooking meat. Health risk assessments were performed based on the resulting exposure to trace elements from such cooking activities. The most abundant elements (significantly different from zero) were Ba (24.4 ug m⁻³) during grilling meat and Ti during heating oil with salt (24.4 ug m⁻³). The health assessment indicates that the cooking with an electric stove with poor ventilation leading to chronic exposures may pose the risk of significant adverse health effects. Carcinogenic risk exceeded the acceptable level (target cancer risk 1 × 10⁻⁶, US EPA 2015) by four orders of magnitude, while non-carcinogenic risk exceeded the safe level (target HQ = 1, US EPA 2015) by a factor of 5–20. Cr and Co were the primary contributors to the highest carcinogenic and non-carcinogenic risks, respectively.
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