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Analysis of changes in air pollution quality and impact of COVID-19 on environmental health in Iran: application of interpolation models and spatial autocorrelation.
2022
Keshtkar, Mostafa | Heidari, Hamed | Moazzeni, Niloofar | Azadi, Hossein
In the global COVID-19 epidemic, humans are faced with a new challenge. The concept of quarantine as a preventive measure has changed human activities in all aspects of life. This challenge has led to changes in the environment as well. The air quality index is one of the immediate concrete parameters. In this study, the actual potential of quarantine effects on the air quality index and related variables in Tehran, the capital of Iran, is assessed, where, first, the data on the pollutant reference concentration for all measuring stations in Tehran, from February 19 to April 19, from 2017 to 2020, are monitored and evaluated. This study investigated the hourly concentrations of six particulate matters (PM), including PM2.5, PM10, and air contaminants such as nitrogen dioxide (NO2), sulfur dioxide (SO2), ozone (O3), and carbon monoxide (CO). Changes in pollution rate during the study period can be due to reduced urban traffic, small industrial activities, and dust mites of urban and industrial origins. Although pollution has declined in most regions during the COVID-19 quarantine period, the PM2.5 rate has not decreased significantly, which might be of natural origins such as dust. Next, the air quality index for the stations is calculated, and then, the interpolation is made by evaluating the root mean square (RMS) of different models. The local and global Moran index indicates that the changes and the air quality index in the study area are clustered and have a high spatial autocorrelation. The results indicate that although the bad air quality is reduced due to quarantine, major changes are needed in urban management to provide favorable conditions. Contaminants can play a role in transmitting COVID-19 as a carrier of the virus. It is suggested that due to the rise in COVID-19 and temperature in Iran, in future studies, the effect of increased temperature on COVID-19 can be assessed. | peer reviewed
Показать больше [+] Меньше [-]Huge quantities of microplastics are “hidden” in the sediment of China's largest urban lake—Tangxun Lake
2022
Shi, Mingming | Li, Rui | Xu, An | Su, Yewang | Hu, Tianpeng | Mao, Yao | Qi, Shihua | Xing, Xinli
Microplastics (MPs) pollution in Tangxun Lake, the largest urban lake in China, was investigated. The average MPs pollution in sediment (1.81 ± 1.75 × 10⁴ items kg⁻¹) is at a high level, while the MPs in lakeshore water (917.77 ± 742.17 items m⁻³) is in the middle to low level compared with existing studies, which is related to the government's protection. Fragments and fibers are the most common shapes in sediment and water, respectively. MPs size <1 mm dominates in the sediment, while the MPs in water has a larger size. The distribution of MPs in the inner lake shows that pellets tend to “hidden” in sediments. Suspected MPs are randomly selected for polymer detection by Micro-Raman microscopy. Polypropylene (PP), polyethylene (PE) and polyethylene terephthalate (PET) are the most common polymer types in water, sediment and atmospheric deposition MPs samples. The input of wastewater, fishery and surrounding human activities are the main sources of MPs in sediment. Atmospheric deposition has a great impact on the distribution of MPs, while the contribution of surface runoff to lake MPs is not remarkable. In addition, MPs in sediments have exceeded the environmental carrying capacity. More attention should be focused on the sediment, where huge amounts of MPs are “hidden”.
Показать больше [+] Меньше [-]Plutonium isotopes in the Qinghai-Tibet Plateau: Sources, distribution, and their environmental behaviors
2022
Zhao, Xue | Hou, Xiaolin | Huang, Zhao | Liu, Heng | Jiang, Huan
Due to the high radiotoxicity in high concentrations, plutonium isotopes have drawn high attentions in the consideration of radiation risk, their sources, level, environmental behaviors, including deposition, retention and migration behaviors. However, such research in the Qinghai-Tibet Plateau is still missing, where is deemed as an environmental sensitive area. ²³⁹,²⁴⁰Pu in surface soil collected from the Qinghai-Tibet Plateau were determined for the first time in this work. The concentrations of ²³⁹,²⁴⁰Pu are in the range of 0.0176–1.95 Bq/kg, falling into the reported ranges in the background areas from the similar latitude belt. The ²⁴⁰Pu/²³⁹Pu atomic ratio range was measured to be 0.146–0.225, which is similar with the global fallout values. Both indicate that the global fallout is the major source of plutonium in this region, and the low plutonium level will not cause any radiation risk so far. Based on the statistical analysis of the possible parameters (organic content, moisture content, average annual precipitation, altitudes, topography and human activity), the large variations of ²³⁹,²⁴⁰Pu concentrations were mainly attributed to the retention process related factors including soil organic content and human activity disturbances. While, the deposition related factors including the average annual precipitation, altitudes, topography made insignificant influence on the spatial distribution of ²³⁹,²⁴⁰Pu concentrations due to the low ²³⁹,²⁴⁰Pu concentrations in atmosphere, less wet deposition amount and insignificant re-suspended amount. The highest ²³⁹,²⁴⁰Pu concentrations of 0.805–1.95 Bq/kg were mainly due to the good retention condition in the sampling sites with higher soil organic content and less human activity disturbances.
Показать больше [+] Меньше [-]Concentrations, homolog profiles, and risk assessment of short- and medium-chain chlorinated paraffins in soil around factories in a non-ferrous metal recycling park
2022
Weng, Jiyuan | Zhang, Peixuan | Gao, Lirong | Zhu, Shuai | Liu, Yang | Qiao, Lin | Zhao, Bin | Liu, Yin | Xu, Ming | Zheng, Minghui
Chlorinated paraffins (CPs) are used as additives in metal processing in the metal smelting industry. Data on CPs in the environment near metal smelting plants are limited. The objectives of this study were to investigate the concentrations and congener profiles of CPs in soil around factories in a non-ferrous metal recycling park located in Hebei, China, and to investigate human exposure to CPs in the soil. The concentrations of short-chain CPs (SCCPs) and medium-chain CPs (MCCPs) were determined by two-dimensional gas chromatography with electron capture negative ionization mass spectrometry. The SCCP and MCCP concentrations in the soil samples were 121–5159 ng/g and 47–6079 ng/g, respectively. Generally, the CP concentrations in soils around the factories were relatively high compared with those near other contaminated sites and in rural and urban areas. There were significant correlations between the MCCP concentrations, some SCCP carbon homologs, and the total organic carbon content (p < 0.05). The major SCCP and MCCP congener groups were C₁₀Cl₆–₇ and C₁₅–₁₆Cl₅, respectively. Hierarchical cluster analysis and principal component analysis indicated that SCCPs and MCCPs in the soil might originate from extreme pressure additives containing CP-42 and CP-52 and CP-containing waste material from the factories. The concentrations in two samples collected near a metal recycling factory posed a moderate risk according to a risk assessment conducted using risk quotients. Further risk assessment showed that the CPs concentrations in soil did not pose significant health risks to either children or adults.
Показать больше [+] Меньше [-]Seasonal distribution of antibiotic resistance genes in the Yellow River water and tap water, and their potential transmission from water to human
2022
Yu, Qiaoling | Feng, Tianshu | Yang, Jiawei | Su, Wanghong | Zhou, Rui | Wang, Yijie | Zhang, Hong | Li, Huan
The prevalence and transmission of antibiotic resistance genes (ARGs) and opportunistic pathogens in water environments can pose great threat to public health. However, the dissemination of ARGs and opportunistic pathogens from water environments to humans has been poorly explored. Here, we employed 16S rRNA gene sequencing and high-throughput quantitative PCR techniques to explore the seasonal distribution of ARGs and opportunistic pathogens in the Yellow River water (source water) and tap water, as well as their relationships with healthy humans at Lanzhou, China. Physiochemical analysis was applied to detect water quality parameters and heavy metal contents. The absolute abundance and diversity of ARGs in the Yellow River and tap water demonstrated distinct seasonal patterns. In winter, the Yellow river water had the highest ARG abundance and diversity, while tap water owned the lowest. Mobile genetic elements (MGEs) were the predominant driver of ARG profiles in both the Yellow river and tap water. Null model analysis showed that ARG assembly in the Yellow River was more influenced by stochastic processes than tap water and this was independent of seasons. Total organic carbon and arsenic contents exhibited positive correlations with many ARGs. Opportunistic pathogens Aeromonas and Pseudomonas may be potential hosts for ARGs. Approximately 80% of detected ARGs were shared between water samples and the human gut. These persistent ARGs could not be entirely eliminated through drinking water treatment processes. Thus, it is crucial to protect sources of tap water from anthropogenic pollution and improve water treatment technologies to reduce the dissemination of ARGs and ensure drinking-water biosafety for human health.
Показать больше [+] Меньше [-]High mortality and high PCDD/Fs exposure among residents downwind of municipal solid waste incinerators: A case study in China
2022
Ji, Guixiang | Chen, Qi | Ding, Zhen | Gu, Jie | Guo, Min | Shi, Lili | Yu, Hao | Sun, Hong
Studies on the human body burden of dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) in populations around municipal solid waste incinerators (MSWIs) in China are limited. The objective of this study was to assess the potential adverse health effects of an 8-year MSWI on the surrounding population and identify possible exposure pathways. We hypothesized that the MSWI would result in different environmental impacts and population health outcomes between upwind and downwind of its 3 km vicinity. We conducted a 10-year retrospective mortality survey on the population surrounding the MSWI. Then, we selected 50 residents aged 50 years or older on each of the upwind and downwind sides of MSWI to test serum PCDD/Fs. Meanwhile, environmental and food exposures to PCDD/Fs were tested for selected residents. The age-adjusted mortality rates were significantly higher for residents downwind than upwind, but no significant difference was found in the standardized mortality ratio before and after the MSWI operation. The toxic equivalents (TEQ) and major congeners of PCDD/Fs were significantly higher in the sera of the downwind residents than in the upwind. The PCDD/Fs in air, soil, dust, and vegetables on the downwind side were not significantly different from those on the upwind side, but the mean concentrations of PCDD/Fs in downwind hen eggs was significantly higher than those from upwind. In conclusion, downwind residents living within 3 km of the MSWI had higher age-adjusted mortality and serum level of PCDD/Fs than upwind residents. This higher mortality rate among downwind residents was not associated with MSWI. However, the higher levels of PCDD/Fs in downwind hen eggs suggest that the downwind population dioxin exposure was related to their location.
Показать больше [+] Меньше [-]Modeling exposure to airborne metals using moss biomonitoring in cemeteries in two urban areas around Paris and Lyon in France
2022
Lequy, Emeline | Meyer, Caroline | Vienneau, Danielle | Berr, Claudine | Goldberg, Marcel | Zins, Marie | Leblond, Sébastien | de Hoogh, Kees | Jacquemin, Bénédicte
Exposure of the general population to airborne metals remains poorly estimated despite the potential health risks. Passive moss biomonitoring can proxy air quality at fine resolution over large areas, mainly in rural areas. We adapted the technique to urban areas to develop fine concentration maps for several metals for Constances cohort's participants. We sampled Grimmia pulvinata in 77 and 51 cemeteries within ∼50 km of Paris and Lyon city centers, respectively. We developed land-use regression models for 14 metals including cadmium, lead, and antimony; potential predictors included the amount of urban, agricultural, forest, and water around cemeteries, population density, altitude, and distance to major roads. We used both kriging with external drift and land use regression followed by residual kriging when necessary to derive concentration maps (500 × 500 m) for each metal and region. Both approaches led to similar results. The most frequent predictors were the amount of urban, agricultural, or forest areas. Depending on the metal, the models explained part of the spatial variability, from 6% for vanadium in Lyon to 84% for antimony in Paris, but mostly between 20% and 60%, with better results for metals emitted by human activities. Moss biomonitoring in cemeteries proves efficient for obtaining airborne metal exposures in urban areas for the most common metals.
Показать больше [+] Меньше [-]Metagenomics highlights the impact of climate and human activities on antibiotic resistance genes in China's estuaries
2022
Zheng, Dongsheng | Yin, Guoyu | Liu, Min | Hou, Lijun | Yang, Yi | Liu, Xinran | Jiang, Yinghui | Chen, Cheng | Wu, Han
Estuarine environments faced with contaminations from coastal zones and the inland are vital sinks of antibiotic resistance genes (ARGs). However, little is known about the temporal-spatial pattern of ARGs and its predominant constraints in estuarine environments. Here, we leveraged metagenomics to investigate ARG profiles from 16 China's estuaries across 6 climate zones in dry and wet seasons, and disentangled their relationships with environmental constraints. Our results revealed that ARG abundance, richness, and diversity in dry season were higher than those in wet season, and ARG abundance exhibited an increasing trend with latitude. The prevalence of ARGs was significantly driven by human activities, mobile gene elements, microbial communities, antibiotic residuals, physicochemical properties, and climatic variables. Among which, climatic variables and human activities ranked the most important factors, contributing 44% and 36% of the total variance of observed ARGs, respectively. The most important climatic variable shaping ARGs is temperature, where increasing temperature is associated with decreased ARGs. Our results highlight that the prevalence of ARGs in estuarine environments would be co-driven by anthropogenic activities and climate, and suggest the dynamics of ARGs under future changing climate and socioeconomic development.
Показать больше [+] Меньше [-]Distribution of rare earth elements (REEs) and their roles in plant growth: A review
2022
Tao, Yue | Shen, Lu | Feng, Chong | Yang, Rongyi | Qu, Jianhua | Ju, Hanxun | Zhang, Ying
The increasing use of rare earth elements (REEs) in various industries has led to a rise in discharge points, thus increasing discharge rates, circulation, and human exposure. Therefore, REEs have received widespread attention as important emerging pollutants. This article thus summarizes and discusses the distribution and occurrence of REEs in the world's soil and water, and briefly introduces current REEs content analysis technology for the examination of different types of samples. Specifically, this review focuses on the impact of REEs on plants, including the distribution and fractionation of REEs in plants and their bioavailability, the effect of REEs on seed germination and growth, the role of REEs in plant resistance, the physiological and biochemical responses of plants in the presence of REEs, including mineral absorption and photosynthesis, as well as a description of the substitution mechanism of REEs competing for Ca in plant cells. Additionally, this article summarizes the potential mechanisms of REEs to activate endocytosis in plants and provides some insights into the mechanisms by which REEs affect endocytosis from a cell and molecular biology perspective. Finally, this article discusses future research prospects and summarizes current scientific findings that could serve as a basis for the development of more sustainable rare earth resource utilization strategies and the assessment of REEs in the environment.
Показать больше [+] Меньше [-]Characterization and biodegradability assessment of water-soluble fraction of oily sludge using stir bar sorptive extraction and GCxGC-TOF MS
2022
Chand, Priyankar | Dutta, Suryendu | Mukherji, Suparna
Percolation of water through oily sludge during storage and handling of the sludge can cause soil and groundwater contamination. In this study, oily sludge from a refinery was equilibrated with water to obtain the water-soluble fraction (WSF) of oily sludge. The WSF had dissolved organic carbon (DOC) of 166 mg/L. Human cell line-based toxicity assay revealed IC₅₀ of 41 mg/L indicating its toxic nature. The predominant compounds in WSF of oily sludge included isomers of methyl, dimethyl and trimethyl quinolines and naphthalenes along with phenol derivatives and other polynuclear aromatic hydrocarbons (PAHs). Biodegradation of WSF of oily sludge was studied using a consortium of Rhodococcus ruber, Bacillus sp. and Bacillus cereus isolated from the refinery sludge. The consortium of the three strains resulted in 70% degradation over 15 days with a first-order degradation rate of 0.161 day⁻¹. Further analysis of the WSF was performed using the stir-bar sorptive extraction (SBSE) followed by GCxGC-TOF MS employing a PDMS Twister. The GCxGC analysis showed that Bacillus cereus was capable of degrading the quinoline, phenol and naphthalene derivatives in WSF of oily sludge at a faster rate compared to pyridine and benzoquinoline derivatives. Quinoline, phenol, biphenyl, naphthalene, pyridine and benzoquinolines derivatives in the WSF of oily sludge were reduced by 87%, 92%, 88%, 77%, 40% and 62%, respectively with respect to the controls. The WSF of oily sludge contained, n-alkanes, ranging from n-C12 to n-C18 which were removed within 2 days of biodegradation.
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