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Biomass burning in eastern Europe during spring 2006 caused high deposition of ammonium in northern Fennoscandia Полный текст
2013
Karlsson, Per Erik | Ferm, Martin | Tømmervik, Hans | Hole, Lars R. | Pihl Karlsson, Gunilla | Ruoho-Airola, Tuija | Aas, Wenche | Hellsten, Sofie | Akselsson, Cecilia | Mikkelsen, Teis Nørgaard | Nihlgård, Bengt
High air concentrations of ammonium were detected at low and high altitude sites in Sweden, Finland and Norway during the spring 2006, coinciding with polluted air from biomass burning in eastern Europe passing over central and northern Fennoscandia. Unusually high values for throughfall deposition of ammonium were detected at one low altitude site and several high altitude sites in north Sweden. The occurrence of the high ammonium in throughfall differed between the summer months 2006, most likely related to the timing of precipitation events. The ammonia dry deposition may have contributed to unusual visible injuries on the tree vegetation in northern Fennoscandia that occurred during 2006, in combination with high ozone concentrations. It is concluded that long-range transport of ammonium from large-scale biomass burning may contribute substantially to the nitrogen load at northern latitudes.
Показать больше [+] Меньше [-]Experimental addition of nitrogen to a whole forest ecosystem at Gårdsjön, Sweden (NITREX): Nitrate leaching during 26 years of treatment Полный текст
2018
Moldan, Filip | Jutterström, Sara E.A-K. | Hruška, Jakub | Wright, Richard F.
Chronic high deposition of nitrogen (N) to forest ecosystems can lead to increased leaching of inorganic N to surface waters, enhancing acidification and eutrophication. For 26 years nitrogen has been added as ammonium nitrate (NH₄NO₃) at 40 kg N ha⁻¹ yr⁻¹ to a whole forested catchment ecosystem at Gårdsjön, Sweden, to experimentally simulate the transition from a N-limited to N-rich state. Over the first 10 years of treatment there was an increasing amount of nitrate (NO₃⁻) and to a lesser extent ammonium (NH₄⁺) lost in runoff, but then N leaching stabilised, and for the subsequent 16 years the fraction of N added lost in runoff remained at 9%. NO₃⁻ concentrations in runoff were low in the summer during the first years of treatment, but now are high throughout the year. High frequency sampling showed that peaks in NO₃⁻ concentrations generally occurred with high discharge, and were enhanced if high discharge coincided with occasions of N addition. Approximately 50% of the added N has gone to the soil. The added N is equivalent to 140 years of ambient N deposition. At current ambient levels of N deposition there thus appears to be no immediate risk of N saturation at this coniferous forest ecosystem, and by inference to other such N-limited forests in Scandinavia.
Показать больше [+] Меньше [-]Chlorinated pesticides and natural brominated anisoles in air at three northern Baltic stations Полный текст
2017
Bidleman, Terry F. | Laudon, Hjalmar | Nygren, Olle | Svanberg, Staffan | Tysklind, Mats
Polyurethane foam (PUF) disk passive samplers were deployed at one inland and two island locations in the Bothnian Bay region of the northern Baltic Sea. Uptake was linear over 81–147 d and a temperature range of −2.6 to 14.2 °C for organochlorine pesticides (OCPs) and current-use pesticides (CUPs) having log KOA ≥9 at ambient temperatures. Partial saturation of the PUF disks occurred for the more volatile OCPs hexachlorocyclohexanes (HCHs) and hexachlorobenzene (HCB), and for bromoanisoles (BAs), which are products of bromophenols released by natural and anthropogenic sources. Correction for nonlinear uptake of these was made using experimentally measured PUF-air partition coefficients. Passive-derived air concentrations of pesticides were uniform over the bay and agreed within a factor of 2 or better with levels determined by active (pumped) sampling at one of the island stations. Levels of OCPs were similar to those reported at background sites in the European and Canadian Arctic and at monitoring stations in the central Baltic and southern Scandinavia, indicating long-range transport. The insecticide chlorpyrifos was 10 times lower at bay stations than in the Canadian Arctic. Insight to sources and processes was gained by examining compound profiles. Fractions Falpha = α-HCH/(α-HCH + γ-HCH) and FTC = trans-chlordane/(trans-chlordane + cis-chlordane) at bay stations were higher than in the Norwegian and Finnish Arctic and similar to those at the southern monitoring stations. Volatilization of chlordanes from Baltic seawater may also modify FTC. Higher FTriBA = 2,4,6-TriBA/(2,4,6-TriBA + 2,4-DiBA) distinguished local volatilization from the Baltic Sea versus lower FTriBA found at the inland site and reported in air on the Norwegian coast, suggesting westerly transport from the Atlantic across Norway and Sweden.
Показать больше [+] Меньше [-]An almost completed pollution-recovery cycle reflected by sediment geochemistry and benthic foraminiferal assemblages in a Swedish–Norwegian Skagerrak fjord Полный текст
2015
Polovodova Asteman, Irina | Hanslik, Daniela | Nordberg, Kjell
During the 20th century Idefjord was considered one of the most polluted marine areas in Scandinavia. For decades it received high discharges from paper/pulp industry, which made it anoxic and extremely polluted by heavy metals and organic contaminants. Today the fjord is close to fulfil a complete pollution-recovery cycle, which is recorded in its sediment archives. Here we report results from five sediment cores studied for TC, C/N, heavy metals and benthic foraminifera. All of the cores have laminations deposited during 1940–1980s and indicative of long-lasting anoxia; high TC and heavy metal content, poor foraminiferal faunas and lack of macrofauna. The upper part of the cores deposited since 1980s shows a gradual pollutant decrease and partial foraminiferal recovery. The majority of foraminiferal species in Idefjord are agglutinated opportunistic and stress-tolerant taxa, which to some extent tolerate hypoxia and are early colonisers of previously disturbed environments. The current study demonstrates a value of benthic foraminiferal stratigraphy as a useful tool in understanding processes driving environmental degradation and recovery of coastal ecosystems.
Показать больше [+] Меньше [-][Animals as carriers of information on the environment [use of mayfly larvae (Baetis rhodani) as indicator species in monitoring of inland water acidification]]
1982
Raddum, G.G. | Fjellheim, A. (Bergen Univ. (Norway). Zoologisk Museum)
Effects of environmental stress on forest crown condition in Europe. Part III: estimation of critical deposition and concentration levels and their exceedances
2000
Vries, W. de | Reinds, G.J. | Klap, J.M. | Leeuwen, E.P. van | Erisman, J.W.
Mapping of Surface Ozone Seasonality and Trends Across Europe During 1997–2006 Through Kriging Interpolation to Observational Data Полный текст
2013
Aggelis, D. | Zanis, P. | Zerefos, C. S. | Bais, A. F. | Nastos, P. T.
Kriging interpolation technique is adapted to create the mapping of surface ozone seasonality and trends across Europe during 1997–2006, based on European Monitoring and Evaluation Programme ground measurements. The climatology, the annual and seasonal trends and the altitude above sea level (asl) dependence were studied as well as the relation with the North Atlantic Oscillation (NAO). The mean seasonal cycle amplitude and seasonal maximum display an increasing gradient from northwest to southeast, with high levels in Austria and eastern Mediterranean. Significantly close to 0 positive trends appear in UK, Slovakia, southern Scandinavia and Austria in winter and autumn. In Northern Hemisphere winter (December–February), about 40 % of near-surface ozone variability in the western edge of Europe may be attributed to circulation changes and ozone precursors’ transport related to NAO.
Показать больше [+] Меньше [-]Water Cover Technology for Reactive Tailings Management: A Case Study of Field Measurement and Model Predictions Полный текст
2011
Kachhwal, Laxmi Kant | Yanful, Ernest K. | Lanteigne, Lisa
Environmentally safe disposal of sulfide-rich reactive mine tailings is one of the major challenges facing the mining industry in Canada, Scandinavia, USA, and many other parts of the world. Placing tailings under a water cover is one of the effective methods to reduce the influx of oxygen to the tailings. Wind-induced turbulence and subsequent resuspension of the tailings, however, are major concerns with this approach. In this paper, a study of wind-induced resuspension at the Shebandowan tailings storage facility, northwestern Ontario, Canada, is discussed. The study compares computer modeling of required water cover depths and resuspended tailings concentrations to observed field data. The calculated minimum water cover depths required to eliminate resuspension were found to be higher than the existing implemented water cover depths in each cell. The predicted resuspended tailings concentrations for the west cell were 6-22 mg/l with an average value of 15 mg/l and, for the east cell, 1-10 mg/l, with an average of 6.0 mg/l. In comparison, optical backscatter sensors, deployed in situ, recorded average resuspended tailings concentration up to 25 mg/l, indicating that the model results were similar to the field-measured values. Results from sediment trap measurements did not show any correlation between the amount of resuspended tailings and water cover depth. Sediment traps collect not only sediments eroded and suspended at the location of deployment but also those that have been transported from elsewhere and redeposited at the trap location. The amount of resuspension occurring at Shebandowan does not raise a major concern because discharge from the tailings area is collected and managed before it reports to the final effluent.
Показать больше [+] Меньше [-]Effects of environmental stress on forest crown condition in Europe. Part I: hypotheses and approach to the study
2000
Vries, W. de | Klap, J.M. | Erisman, J.W.
Determinants of maternal and fetal exposure and temporal trends of perfluorinated compounds Полный текст
2013
Ode, Amanda | Rylander, Lars | Lindh, Christian H. | Källén, Karin | Jönsson, Bo A. G. | Gustafsson, Peik | Olofsson, Per | Ivarsson, Sten A. | Rignell-Hydbom, Anna
In recent years, some perfluorinated compounds (PFCs) have been identified as potentially hazardous substances which are harmful to the environment and human health. According to limited data, PFC levels in humans could be influenced by several determinants. However, the findings are inconsistent. In the present study, perfluorooctane sulfonate (PFOS), perfluorooctanoic acid (PFOA), and perfluorononanoic acid (PFNA) were measured in paired maternal and cord serum samples (N = 237) collected between 1978 and 2001 in Southern Sweden to study the relationship between these and to investigate several potential determinants of maternal and fetal exposure to PFCs. Time trends of PFCs in Swedish women were also evaluated. The study is a part of the Fetal Environment and Neurodevelopment Disorders in Epidemiological Research project. PFOS, PFOA, and PFNA levels (median) were higher in maternal serum (15, 2.1, and 0.24 ng/ml, respectively) than in cord serum (6.5, 1.7, and 0.20 ng/ml, respectively). PFC levels were among the highest in women originating from the Nordic countries and the lowest in women from the Middle East, North Africa, and sub-Saharan Africa. Multiparous women had lower serum PFOA levels (1.7 ng/ml) than primiparous women (2.4 ng/ml). Maternal age, body mass index, cotinine levels, and whether women carried male or female fetuses did not affect serum PFC concentrations. Umbilical cord serum PFC concentrations showed roughly similar patterns as the maternal except for the gestational age where PFC levels increased with advancing gestational age. PFOS levels increased during the study period in native Swedish women. In summary, PFOS levels tend to increase while PFOA and PFNA levels were unchanged between 1978 and 2001 in our study population. Our results demonstrate that maternal country of origin, parity, and gestational age might be associated with PFC exposure.
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